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Dielectric catastrophe at the Wigner-Mott transition in a moire superlattice.

ABSTRACT: The bandwidth-tuned Wigner-Mott transition is an interaction-driven phase transition from a generalized Wigner crystal to a Fermi liquid. Because the transition is generally accompanied by both magnetic and charge-order instabilities, it remains unclear if a continuous Wigner-Mott transition exists. Here, we demonstrate bandwidth-tuned metal-insulator transitions at fixed fractional fillings of a MoSe₂/WS₂ moiré superlattice. The bandwidth is controlled by an out-of-plane electric field. The dielectric response is probed optically with the 2s exciton in a remote WSe₂ sensor layer. The exciton spectral weight is negligible for the metallic state with a large negative dielectric constant. It continuously vanishes when the transition is approached from the insulating side, corresponding to a diverging dielectric constant or a 'dielectric catastrophe' driven by the critical charge dynamics near the transition. Our results support the scenario of continuous Wigner-Mott transitions in two-dimensional triangular lattices and stimulate future explorations of exotic quantum phases in their vicinities.

SUBMITTER: Tang Y

PROVIDER: S-EPMC9314335 | biostudies-literature |

REPOSITORIES: biostudies-literature

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Quadrupolar excitons and hybridized interlayer Mott insulator in a trilayer moire superlattice.

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