Dataset Information

Multifunctional SiC@SiO₂ Nanofiber Aerogel with Ultrabroadband Electromagnetic Wave Absorption.

ABSTRACT: Traditional ceramic materials are generally brittle and not flexible with high production costs, which seriously hinders their practical applications. Multifunctional nanofiber ceramic aerogels are highly desirable for applications in extreme environments, however, the integration of multiple functions in their preparation is extremely challenging. To tackle these challenges, we fabricated a multifunctional SiC@SiO₂ nanofiber aerogel (SiC@SiO₂ NFA) with a three-dimensional (3D) porous cross-linked structure through a simple chemical vapor deposition method and subsequent heat-treatment process. The as-prepared SiC@SiO₂ NFA exhibits an ultralow density (~ 11 mg cm^- 3), ultra-elastic, fatigue-resistant and refractory performance, high temperature thermal stability, thermal insulation properties, and significant strain-dependent piezoresistive sensing behavior. Furthermore, the SiC@SiO₂ NFA shows a superior electromagnetic wave absorption performance with a minimum refection loss (RL_min) value of - 50.36 dB and a maximum effective absorption bandwidth (EAB_max) of 8.6 GHz. The successful preparation of this multifunctional aerogel material provides a promising prospect for the design and fabrication of the cutting-edge ceramic materials.

SUBMITTER: Song L

PROVIDER: S-EPMC9334492 | biostudies-literature | 2022 Jul

REPOSITORIES: biostudies-literature

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Publications

Multifunctional SiC@SiO2 Nanofiber Aerogel with Ultrabroadband Electromagnetic Wave Absorption.

Song Limeng L Zhang Fan F Chen Yongqiang Y Guan Li L Zhu Yanqiu Y Chen Mao M Wang Hailong H Putra Budi Riza BR Zhang Rui R Fan Bingbing B

Nano-micro letters 20220728 1

Traditional ceramic materials are generally brittle and not flexible with high production costs, which seriously hinders their practical applications. Multifunctional nanofiber ceramic aerogels are highly desirable for applications in extreme environments, however, the integration of multiple functions in their preparation is extremely challenging. To tackle these challenges, we fabricated a multifunctional SiC@SiO2 nanofiber aerogel (SiC@SiO2 NFA) with a three-dimensional ...[more]

PMID: 35900619

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Project description:The fabrication of superadsorbent for dye adsorption is a hot research area at present. However, the development of low-cost and highly efficient superadsorbents against toxic textile dyes is still a big challenge. Here, we fabricated hydrophobic cellulose nanofiber aerogels from cellulose nanofibers through an eco-friendly silanization reaction in liquid phase, which is an extremely efficient, rapid, cheap, and environmentally friendly procedure. Moreover, the demonstrated eco-friendly silanization technique is easy to commercialize at the industrial level. Most of the works that have reported on the hydrophobic cellulose nanofiber aerogels explored their use for the elimination of oil from water. The key novelty of the present work is that the demonstrated hydrophobic cellulose nanofibers aerogels could serve as superadsorbents against toxic textile dyes such as crystal violet dye from water and insulating materials for building applications. Here, we make use of the possible hydrophobic interactions between silane-modified cellulose nanofiber aerogel and crystal violet dye for the removal of the crystal violet dye from water. With a 10 mg/L of crystal violet (CV) aqueous solution, the silane-modified cellulose nanofiber aerogel showed a high adsorption capacity value of 150 mg/g of the aerogel. The reason for this adsorption value was due to the short-range hydrophobic interaction between the silane-modified cellulose nanofiber aerogel and the hydrophobic domains in crystal violet dye molecules. Additionally, the fabricated silane-modified cellulose nanofiber hydrophobic aerogels exhibited a lower thermal conductivity value of 0.037 W·m-1 K-1, which was comparable to and lower than the commercial insulators such as mineral wools (0.040 W·m-1 K-1) and polystyrene foams (0.035 W·m-1 K-1). We firmly believe that the demonstrated silane-modified cellulose nanofiber aerogel could yield an eco-friendly adsorbent that is agreeable to adsorbing toxic crystal violet dyes from water as well as active building thermal insulators.

Dataset Information

Multifunctional SiC@SiO₂ Nanofiber Aerogel with Ultrabroadband Electromagnetic Wave Absorption.

Publications

Multifunctional SiC@SiO<sub>2</sub> Nanofiber Aerogel with Ultrabroadband Electromagnetic Wave Absorption.

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