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Correlation-driven electronic nematicity in the Dirac semimetal BaNiS2.


ABSTRACT: In BaNiS2, a Dirac nodal line band structure exists within a two-dimensional Ni square lattice system, in which significant electronic correlation effects are anticipated. Using scanning tunneling microscopy (STM), we discover signs of correlated-electron behavior, namely electronic nematicity appearing as a pair of C2-symmetry striped patterns in the local density-of-states at ∼60 meV above the Fermi energy. In observations of quasiparticle interference, as well as identifying scattering between Dirac cones, we find that the striped patterns in real space stem from a lifting of degeneracy among electron pockets at the Brillouin zone boundary. We infer a momentum-dependent energy shift with d-form factor, which we model numerically within a density wave (DW) equation framework that considers spin-fluctuation-driven nematicity. This suggests an unusual mechanism driving the nematic instability, stemming from only a small perturbation to the Fermi surface, in a system with very low density of states at the Fermi energy. The Dirac points lie at nodes of the d-form factor and are almost unaffected by it. These results highlight BaNiS2 as a unique material in which Dirac electrons and symmetry-breaking electronic correlations coexist.

SUBMITTER: Butler CJ 

PROVIDER: S-EPMC9894198 | biostudies-literature | 2022 Dec

REPOSITORIES: biostudies-literature

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Correlation-driven electronic nematicity in the Dirac semimetal BaNiS<sub>2</sub>.

Butler Christopher John CJ   Kohsaka Yuhki Y   Yamakawa Youichi Y   Bahramy Mohammad Saeed MS   Onari Seiichiro S   Kontani Hiroshi H   Hanaguri Tetsuo T   Shamoto Shinichi S  

Proceedings of the National Academy of Sciences of the United States of America 20221202 49


In BaNiS<sub>2</sub>, a Dirac nodal line band structure exists within a two-dimensional Ni square lattice system, in which significant electronic correlation effects are anticipated. Using scanning tunneling microscopy (STM), we discover signs of correlated-electron behavior, namely electronic nematicity appearing as a pair of <i>C</i><sub>2</sub>-symmetry striped patterns in the local density-of-states at ∼60 meV above the Fermi energy. In observations of quasiparticle interference, as well as  ...[more]

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