Browse
Submit Data
Databases
API
Help

Dataset Information

0 Views

0 Connections

0 Citations

0 Reanalyses

0 Downloads

Omics score: 0

Distinct itinerant spin-density waves and local-moment antiferromagnetism in an intermetallic ErPd2Si2 single crystal.

ABSTRACT: Identifying the nature of magnetism, itinerant or localized, remains a major challenge in condensed-matter science. Purely localized moments appear only in magnetic insulators, whereas itinerant moments more or less co-exist with localized moments in metallic compounds such as the doped-cuprate or the iron-based superconductors, hampering a thorough understanding of the role of magnetism in phenomena like superconductivity or magnetoresistance. Here we distinguish two antiferromagnetic modulations with respective propagation wave vectors at Q± = (H ± 0.557(1), 0, L ± 0.150(1)) and QC = (H ± 0.564(1), 0, L), where (H, L) are allowed Miller indices, in an ErPd2Si2 single crystal by neutron scattering and establish their respective temperature- and field-dependent phase diagrams. The modulations can co-exist but also compete depending on temperature or applied field strength. They couple differently with the underlying lattice albeit with associated moments in a common direction. The Q± modulation may be attributed to localized 4f moments while the QC correlates well with itinerant conduction bands, supported by our transport studies. Hence, ErPd2Si2 represents a new model compound that displays clearly-separated itinerant and localized moments, substantiating early theoretical predictions and providing a unique platform allowing the study of itinerant electron behavior in a localized antiferromagnetic matrix.

SUBMITTER: Li HF

PROVIDER: S-EPMC4302317 | biostudies-other | 2015

REPOSITORIES: biostudies-other

ACCESS DATA

Json Xml

Similar Datasets

The dipole moment of the spin density as a local indicator for phase transitions.

Project description:The intra-atomic magnetic dipole moment - frequently called ⟨Tz⟩ term - plays an important role in the determination of spin magnetic moments by x-ray absorption spectroscopy for systems with nonspherical spin density distributions. In this work, we present the dipole moment as a sensitive monitor to changes in the electronic structure in the vicinity of a phase transiton. In particular, we studied the dipole moment at the Fe(2+) and Fe(3+) sites of magnetite as an indicator for the Verwey transition by a combination of x-ray magnetic circular dichroism and density functional theory. Our experimental results prove that there exists a local change in the electronic structure at temperatures above the Verwey transition correlated to the known spin reorientation. Furthermore, it is shown that measurement of the dipole moment is a powerful tool to observe this transition in small magnetite nanoparticles for which it is usually screened by blocking effects in classical magnetometry.

| S-EPMC4104392 | biostudies-literature

Chirality locking charge density waves in a chiral crystal.

Project description:In Weyl semimetals, charge density wave (CDW) order can spontaneously break the chiral symmetry, gap out the Weyl nodes, and drive the material into the axion insulating phase. Investigations have however been limited since CDWs are rarely seen in Weyl semimetals. Here, using scanning tunneling microscopy/spectroscopy (STM/S), we report the discovery of a novel unidirectional CDW order on the (001) surface of chiral crystal CoSi - a unique Weyl semimetal with unconventional chiral fermions. The CDW is incommensurate with both lattice momentum and crystalline symmetry directions, and exhibits an intra unit cell π phase shift in the layer stacking direction. The tunneling spectrum shows a particle-hole asymmetric V-shaped energy gap around the Fermi level that modulates spatially with the CDW wave vector. Combined with first-principle calculations, we identify that the CDW is locked to the crystal chirality and is related by a mirror reflection between the two enantiomers of the chiral crystal. Our findings reveal a novel correlated topological quantum state in chiral CoSi crystals and raise the potential for exploring the unprecedented physical behaviors of unconventional chiral fermions.

| S-EPMC9133074 | biostudies-literature

Directional Excitation of a High-Density Magnon Gas Using Coherently Driven Spin Waves.

Project description:Controlling magnon densities in magnetic materials enables driving spin transport in magnonic devices. We demonstrate the creation of large, out-of-equilibrium magnon densities in a thin-film magnetic insulator via microwave excitation of coherent spin waves and subsequent multimagnon scattering. We image both the coherent spin waves and the resulting incoherent magnon gas using scanning-probe magnetometry based on electron spins in diamond. We find that the gas extends unidirectionally over hundreds of micrometers from the excitation stripline. Surprisingly, the gas density far exceeds that expected for a boson system following a Bose-Einstein distribution with a maximum value of the chemical potential. We characterize the momentum distribution of the gas by measuring the nanoscale spatial decay of the magnetic stray fields. Our results show that driving coherent spin waves leads to a strong out-of-equilibrium occupation of the spin-wave band, opening new possibilities for controlling spin transport and magnetic dynamics in target directions.

| S-EPMC8517981 | biostudies-literature

Spin-orbit torque-driven propagating spin waves.

Project description:Spin-orbit torque (SOT) can drive sustained spin wave (SW) auto-oscillations in a class of emerging microwave devices known as spin Hall nano-oscillators (SHNOs), which have highly nonlinear properties governing robust mutual synchronization at frequencies directly amenable to high-speed neuromorphic computing. However, all demonstrations have relied on localized SW modes interacting through dipolar coupling and/or direct exchange. As nanomagnonics requires propagating SWs for data transfer and additional computational functionality can be achieved using SW interference, SOT-driven propagating SWs would be highly advantageous. Here, we demonstrate how perpendicular magnetic anisotropy can raise the frequency of SOT-driven auto-oscillations in magnetic nanoconstrictions well above the SW gap, resulting in the efficient generation of field and current tunable propagating SWs. Our demonstration greatly extends the functionality and design freedom of SHNOs, enabling long-range SOT-driven SW propagation for nanomagnonics, SW logic, and neuromorphic computing, directly compatible with CMOS technology.

| S-EPMC6868678 | biostudies-literature

Nanometre-scale probing of spin waves using single-electron spins.

Project description:Pushing the frontiers of condensed-matter magnetism requires the development of tools that provide real-space, few-nanometre-scale probing of correlated-electron magnetic excitations under ambient conditions. Here we present a practical approach to meet this challenge, using magnetometry based on single nitrogen-vacancy centres in diamond. We focus on spin-wave excitations in a ferromagnetic microdisc, and demonstrate local, quantitative and phase-sensitive detection of the spin-wave magnetic field at ?50?nm from the disc. We map the magnetic-field dependence of spin-wave excitations by detecting the associated local reduction in the disc's longitudinal magnetization. In addition, we characterize the spin-noise spectrum by nitrogen-vacancy spin relaxometry, finding excellent agreement with a general analytical description of the stray fields produced by spin-spin correlations in a 2D magnetic system. These complementary measurement modalities pave the way towards imaging the local excitations of systems such as ferromagnets and antiferromagnets, skyrmions, atomically assembled quantum magnets, and spin ice.

| S-EPMC4918315 | biostudies-other

The first moment of income density functions and estimation of single-parametric Lorenz curves.

Project description:This paper discusses the first moment, i.e., the mean income point, of income density functions and the estimation of single-parametric Lorenz curves. The mean income point is implied by an income density function and associated with a single-parametric Lorenz function. The boundary of the mean income point can show the flexibility of a parametric Lorenz function. I minimize the sum of squared errors in fitting both grouped income data and the mean income point and identify the best parametric Lorenz function using a large panel dataset. I find that each parametric Lorenz function may do a better job than others in fitting particular grouped data; however, a zero- and unit-modal single-parametric Lorenz function is identified to be the best of eight typical optional functions in fitting most (666 out of 969) observations of a large panel dataset. I perform a Monte Carlo simulation as a robustness check of the empirical estimation.

| S-EPMC9231794 | biostudies-literature

Intrinsic spin of elastic waves.

Project description:Unveiling spins of physical systems usually gives people a fundamental understanding of the geometrical properties of waves from classical to quantum aspects. A great variety of research has shown that transverse waves can possess nontrivial spins and spin-related properties naturally. However, until now, we still lack essential physical insights about the spin nature of longitudinal waves. Here, demonstrated by elastic waves, we uncover spins for longitudinal waves and the mixed longitudinal-transverse waves that play essential roles in spin-momentum locking. Based on this spin perspective, several abnormal phenomena beyond pure transverse waves are attributed to the hybrid spin induced by mixed longitudinal-transverse waves. The unique hybrid spin reveals the complex spin essence in elastic waves and advances our understanding about their fundamental geometrical properties. We also show that these spin-dependent phenomena can be exploited to control the wave propagation, such as nonsymmetric elastic wave excitation by spin pairs, a unidirectional Rayleigh wave, and spin-selected elastic wave routing. These findings are generally applicable for wave cases with longitudinal and transverse components.

| S-EPMC6176628 | biostudies-literature

Temperature induced spin switching in SmFeO3 single crystal.

Project description:The prospect of controlling the magnetization (M) of a material is of great importance from the viewpoints of fundamental physics and future applications of emerging spintronics. A class of rare-earth orthoferrites RFeO3 (R is rare-earth element) materials exhibit striking physical properties of spin switching and magnetization reversal induced by temperature and/or applied magnetic field. Furthermore, due to the novel magnetic, magneto-optic and multiferroic properties etc., RFeO3 materials are attracting more and more interests in recent years. We have prepared and investigated a prototype of RFeO3 materials, namely SmFeO3 single-crystal. And we report magnetic measurements upon both field cooling (FC) and zero-field cooling (ZFC) of the sample, as a function of temperature and applied magnetic field. The central findings of this study include that the magnetization of single-crystal SmFeO3 can be switched by temperature, and tuning the magnitude of applied magnetic field allows us to realize such spin switching even at room temperature.

| S-EPMC4121608 | biostudies-other

Tuning Fe Spin Moment in Fe-N-C Catalysts to Climb the Activity Volcano via a Local Geometric Distortion Strategy.

Project description:As the most promising alternative to platinum-based catalysts for cathodic oxygen reduction reaction (ORR) in proton exchange membrane fuel cells, further performance enhancement of Fe-N-C catalysts is highly expected to promote their wide application. In Fe-N-C catalysts, the single Fe atom forms a square-planar configuration with four adjacent N atoms (D4h symmetry). Breaking the D4h symmetry of the FeN4 active center provides a new route to boost the activity of Fe-N-C catalysts. Herein, for the first time, the deformation of the square-planar coordination of FeN4 moiety achieved by introducing chalcogen oxygen groups (XO2 , X = S, Se, Te) as polar functional groups in the Fe-N-C catalyst is reported. The theoretical and experimental results demonstrate that breaking the D4h symmetry of FeN4 results in the rearrangement of Fe 3d electrons and increases spin moment of Fe centers. The efficient spin state manipulation optimizes the adsorption energetics of ORR intermediates, thereby significantly promoting the intrinsic ORR activity of Fe-N-C catalysts, among which the SeO2 modified catalyst lies around the peak of the ORR volcano plot. This work provides a new strategy to tune the local coordination and thus the electronic structure of single-atom catalysts.

| S-EPMC9631079 | biostudies-literature

Photoinduced spin dynamics in a uniaxial intermetallic heterostructure [Formula: see text].

Project description:Intermetallic heterostructures of rare-earth and transition metals exhibit physical properties prospective for various applications. These structures combine giant magnetostriction, controllable magnetic anisotropy, magneto-optical activity and allow spin reorientation transitions (SRT) induced by magnetic field at room temperature. Here, we present the results of a study of spin dynamics induced by ultrafast optical excitation in the [Formula: see text] heterostructure. The time dependence of the light polarization rotation excited by a pump optical pulse with a duration of 35 fs was measured in the total range of the SRT created by external DC magnetic field. We found hysteretic dependence of the polarization rotation on magnetizing field that is specific for spin dynamics near SRT. Enhancement of the rotation is observed in the critical points of the SRT and near the points of magnetization switch from metastable to stable spin states. In the time-domain, two characteristic delays of 20 ps and 200 ps were found, corresponding to the maximum deviation of the light polarization after excitation. The first is explained by the precession motion of spins out of the plane of the structure. The latter is accounted for the spin in-plane deviation from its initial position and thermal relaxation of the anisotropy.

| S-EPMC7519156 | biostudies-literature

OmicsDI is part of the ELIXIR infrastructure

OmicsDI is an Elixir interoperability service. Learn more ›

Tweets

OmicsDI Databases

PRIDE
PeptideAtlas
MassIVE
JPOST Repository
Physiome Model Repository

EGA
EVA
ENA
LINCS
PAXDB
Cell Collective

MetaboLights
Metabolomics Workbench
MetabolomeExpress
GNPS
BioModels
FAIRDOMHub

ArrayExpress
dbGaP
ExpressionAtlas
GEO
NODE

Information

Databases
Help
API
Contact us
Code on GitHub
Terms of use
Submit Data