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Single-step ambient-air synthesis of graphene from renewable precursors as electrochemical genosensor.


ABSTRACT: Thermal chemical vapour deposition techniques for graphene fabrication, while promising, are thus far limited by resource-consuming and energy-intensive principles. In particular, purified gases and extensive vacuum processing are necessary for creating a highly controlled environment, isolated from ambient air, to enable the growth of graphene films. Here we exploit the ambient-air environment to enable the growth of graphene films, without the need for compressed gases. A renewable natural precursor, soybean oil, is transformed into continuous graphene films, composed of single-to-few layers, in a single step. The enabling parameters for controlled synthesis and tailored properties of the graphene film are discussed, and a mechanism for the ambient-air growth is proposed. Furthermore, the functionality of the graphene is demonstrated through direct utilization as an electrode to realize an effective electrochemical genosensor. Our method is applicable to other types of renewable precursors and may open a new avenue for low-cost synthesis of graphene films.

SUBMITTER: Seo DH 

PROVIDER: S-EPMC5290271 | biostudies-other | 2017 Jan

REPOSITORIES: biostudies-other

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Single-step ambient-air synthesis of graphene from renewable precursors as electrochemical genosensor.

Seo Dong Han DH   Pineda Shafique S   Fang Jinghua J   Gozukara Yesim Y   Yick Samuel S   Bendavid Avi A   Lam Simon Kwai Hung SK   Murdock Adrian T AT   Murphy Anthony B AB   Han Zhao Jun ZJ   Ostrikov Kostya Ken KK  

Nature communications 20170130


Thermal chemical vapour deposition techniques for graphene fabrication, while promising, are thus far limited by resource-consuming and energy-intensive principles. In particular, purified gases and extensive vacuum processing are necessary for creating a highly controlled environment, isolated from ambient air, to enable the growth of graphene films. Here we exploit the ambient-air environment to enable the growth of graphene films, without the need for compressed gases. A renewable natural pre  ...[more]

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