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Ultrafast nonlinear optical response in solution dispersions of black phosphorus.

ABSTRACT: We report the spatial self-phase modulation (SSPM) effect for solution dispersions of black phosphorus (BP). The experimental results suggest that this concentration-dependent coherent light diffraction is due to the ultrafast and large third-order optical nonlinearity of BP. The third-order nonlinear susceptibility of BP has been simply obtained about 10-19?m2/V2 by analyzing the experimental results. The fast relaxation time during dynamic relaxation is obtained as 0.13?ps. Our experimental results imply novel potential application of BP in ultrafast nonlinear phase modulation devices based on their nonlinear optical response.

SUBMITTER: Miao L

PROVIDER: S-EPMC5469804 | biostudies-other | 2017 Jun

REPOSITORIES: biostudies-other

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Ultrafast nonlinear optical response in solution dispersions of black phosphorus.

Miao Lili L Shi Bingxin B Yi Jun J Jiang Yaqin Y Zhao Chujun C Wen Shuangchun S

Scientific reports 20170613 1

We report the spatial self-phase modulation (SSPM) effect for solution dispersions of black phosphorus (BP). The experimental results suggest that this concentration-dependent coherent light diffraction is due to the ultrafast and large third-order optical nonlinearity of BP. The third-order nonlinear susceptibility of BP has been simply obtained about 10-19 m2/V2 by analyzing the experimental results. The fast relaxation time during dynamic relaxation is obtaine ...[more]

PMID: 28611448

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