Ontology highlight
ABSTRACT:
SUBMITTER: von Conta A
PROVIDER: S-EPMC6082858 | biostudies-other | 2018 Aug
REPOSITORIES: biostudies-other
von Conta A A Tehlar A A Schletter A A Arasaki Y Y Takatsuka K K Wörner H J HJ
Nature communications 20180808 1
Time-resolved photoelectron spectroscopy (TRPES) is a useful approach to elucidate the coupled electronic-nuclear quantum dynamics underlying chemical processes, but has remained limited by the use of low photon energies. Here, we demonstrate the general advantages of XUV-TRPES through an application to NO<sub>2</sub>, one of the simplest species displaying the complexity of a non-adiabatic photochemical process. The high photon energy enables ionization from the entire geometrical configuration ...[more]