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Twirling and Spontaneous Symmetry Breaking of Domain Wall Networks in Lattice-Reconstructed Heterostructures of Two-Dimensional Materials.


ABSTRACT: Lattice relaxation in twistronic bilayers with close lattice parameters and almost perfect crystallographic alignment of the layers results in the transformation of the moiré pattern into a sequence of preferential stacking domains and domain wall networks. Here, we show that reconstructed moiré superlattices of the perfectly aligned heterobilayers of same chalcogen transition metal dichalcogenides have broken-symmetry structures featuring twisted nodes ("twirls") of domain wall networks. The analysis of twist-angle dependence of strain characteristics for the broken-symmetry structures shows that the formation of twirl reduces the amount of hydrostatic strain around the nodes, potentially weakening their influence on the band edge energies of electrons and holes.

SUBMITTER: Kaliteevski MA 

PROVIDER: S-EPMC10571146 | biostudies-literature | 2023 Oct

REPOSITORIES: biostudies-literature

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Twirling and Spontaneous Symmetry Breaking of Domain Wall Networks in Lattice-Reconstructed Heterostructures of Two-Dimensional Materials.

Kaliteevski Mikhail A MA   Enaldiev Vladimir V   Fal'ko Vladimir I VI  

Nano letters 20231002 19


Lattice relaxation in twistronic bilayers with close lattice parameters and almost perfect crystallographic alignment of the layers results in the transformation of the moiré pattern into a sequence of preferential stacking domains and domain wall networks. Here, we show that reconstructed moiré superlattices of the perfectly aligned heterobilayers of same chalcogen transition metal dichalcogenides have broken-symmetry structures featuring twisted nodes ("twirls") of domain wall networks. The an  ...[more]

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