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Tuning Fluorescence Direction with Plasmonic Metal-Dielectric- Metal Substrates.


ABSTRACT: Controlling the emission properties of fluorophores is essential for improving the performance of fluorescence-based techniques in modern biochemical research, medical diagnosis, and sensing. Fluorescence emission is isotropic in nature, which makes it difficult to capture more than a small fraction of the total emission. Metal- dielectric-metal (MDM) substrates, discussed in this Letter, convert isotropic fluorescence into beaming emission normal to the substrate. This improves fluorescence collection efficiency and also opens up new avenues for a wide range of fluorescence-based applications. We suggest that MDM substrates can be readily adapted for multiple uses, such as in microarray formats, for directional fluorescence studies of multiple probes or for molecule-specific sensing with a high degree of spatial control over the fluorescence emission. SECTION:Physical Processes in Nanomaterials and Nanostructures.

SUBMITTER: Choudhury SD 

PROVIDER: S-EPMC3762509 | biostudies-literature | 2013

REPOSITORIES: biostudies-literature

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Tuning Fluorescence Direction with Plasmonic Metal-Dielectric- Metal Substrates.

Choudhury Sharmistha Dutta SD   Badugu Ramachandram R   Nowaczyk Kazimierz K   Ray Krishanu K   Lakowicz Joseph R JR  

The journal of physical chemistry letters 20130101 1


Controlling the emission properties of fluorophores is essential for improving the performance of fluorescence-based techniques in modern biochemical research, medical diagnosis, and sensing. Fluorescence emission is isotropic in nature, which makes it difficult to capture more than a small fraction of the total emission. Metal- dielectric-metal (MDM) substrates, discussed in this Letter, convert isotropic fluorescence into beaming emission normal to the substrate. This improves fluorescence col  ...[more]

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