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In situ sediment treatment using activated carbon: a demonstrated sediment cleanup technology.

ABSTRACT: This paper reviews general approaches for applying activated carbon (AC) amendments as an in situ sediment treatment remedy. In situ sediment treatment involves targeted placement of amendments using installation options that fall into two general approaches: 1) directly applying a thin layer of amendments (which potentially incorporates weighting or binding materials) to surface sediment, with or without initial mixing; and 2) incorporating amendments into a premixed, blended cover material of clean sand or sediment, which is also applied to the sediment surface. Over the past decade, pilot- or full-scale field sediment treatment projects using AC-globally recognized as one of the most effective sorbents for organic contaminants-were completed or were underway at more than 25 field sites in the United States, Norway, and the Netherlands. Collectively, these field projects (along with numerous laboratory experiments) have demonstrated the efficacy of AC for in situ treatment in a range of contaminated sediment conditions. Results from experimental studies and field applications indicate that in situ sequestration and immobilization treatment of hydrophobic organic compounds using either installation approach can reduce porewater concentrations and biouptake significantly, often becoming more effective over time due to progressive mass transfer. Certain conditions, such as use in unstable sediment environments, should be taken into account to maximize AC effectiveness over long time periods. In situ treatment is generally less disruptive and less expensive than traditional sediment cleanup technologies such as dredging or isolation capping. Proper site-specific balancing of the potential benefits, risks, ecological effects, and costs of in situ treatment technologies (in this case, AC) relative to other sediment cleanup technologies is important to successful full-scale field application. Extensive experimental studies and field trials have shown that when applied correctly, in situ treatment via contaminant sequestration and immobilization using a sorbent material such as AC has progressed from an innovative sediment remediation approach to a proven, reliable technology.

SUBMITTER: Patmont CR

PROVIDER: S-EPMC4409844 | biostudies-literature | 2015 Apr

REPOSITORIES: biostudies-literature

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In situ sediment treatment using activated carbon: a demonstrated sediment cleanup technology.

Patmont Clayton R CR Ghosh Upal U LaRosa Paul P Menzie Charles A CA Luthy Richard G RG Greenberg Marc S MS Cornelissen Gerard G Eek Espen E Collins John J Hull John J Hjartland Tore T Glaza Edward E Bleiler John J Quadrini James J

Integrated environmental assessment and management 20150106 2

This paper reviews general approaches for applying activated carbon (AC) amendments as an in situ sediment treatment remedy. In situ sediment treatment involves targeted placement of amendments using installation options that fall into two general approaches: 1) directly applying a thin layer of amendments (which potentially incorporates weighting or binding materials) to surface sediment, with or without initial mixing; and 2) incorporating amendments into a premixed, blended cover material of ...[more]

PMID: 25323491

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Project description:Thin-layer capping using activated carbon has been described as a cost-effective in situ sediment remediation method for organic contaminants. We compared the capping efficiency of powdered activated carbon (PAC) against granular activated carbon (GAC) using contaminated sediment from Oskarshamn harbor, Sweden. The effects of resuspension on contaminant retention and cap integrity were also studied. Intact sediment cores were collected from the outer harbor and brought to the laboratory. Three thin-layer caps, consisting of PAC or GAC mixed with clay or clay only, were added to the sediment surface. Resuspension was created using a motor-driven paddle to simulate propeller wash from ship traffic. Passive samplers were placed in the sediment and in the water column to measure the sediment-to-water release of polycyclic aromatic hydrocarbons (PAHs), polychlorinated biphenyls (PCBs), and metals. Our results show that a thin-layer cap with PAC reduced sediment-to-water fluxes of PCBs by 57% under static conditions and 91% under resuspension. Thin-layer capping with GAC was less effective than PAC but reduced fluxes of high-molecular weight PAHs. Thin-layer capping with activated carbon was less effective at retaining metals, except for Cd, the release of which was significantly reduced by PAC. Resuspension generally decreased water concentrations of dissolved cationic metals, perhaps because of sorption to suspended sediment particles. Sediment resuspension in treatments without capping increased fluxes of PCBs with log octanol-water partitioning coefficient (KOW ) > 7 and PAHs with log KOW of 5-6, but resuspension reduced PCB and PAH fluxes through the PAC thin-layer cap. Overall, PAC performed better than GAC, but adverse effects on the benthic community and transport of PAC to nontarget areas are drawbacks that favor the use of GAC. Environ Toxicol Chem 2022;41:1096-1110. © 2022 The Authors. Environmental Toxicology and Chemistry published by Wiley Periodicals LLC on behalf of SETAC.

Dataset Information

In situ sediment treatment using activated carbon: a demonstrated sediment cleanup technology.

Publications

In situ sediment treatment using activated carbon: a demonstrated sediment cleanup technology.

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