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Screened moments and extrinsic in-gap states in samarium hexaboride.


ABSTRACT: Samarium hexaboride (SmB6) is a Kondo insulator, with a narrow gap due to hybridization between localized and conduction electrons. Despite being an insulator, many samples show metal-like properties. Rare-earth purification is exceedingly difficult, and nominally pure samples may contain 2% or more of impurities. Here to determine the effects of rare-earth doping on SmB6, we synthesized and probed a series of gadolinium-doped samples. We found a relationship between specific heat and impurity moment screening which scales systematically. Consistent with this finding, our neutron scattering experiments of a high purity sample of doubly isotopic 154Sm11B6 show no intrinsic excitations below the well-established 13?meV spin-exciton. The result of introducing impurities into a Kondo insulator is incompletely understood, but it is clear from our measurements that there is a systematic relationship between rare-earth impurities and metal-like properties in SmB6.

SUBMITTER: Fuhrman WT 

PROVIDER: S-EPMC5906653 | biostudies-literature | 2018 Apr

REPOSITORIES: biostudies-literature

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Screened moments and extrinsic in-gap states in samarium hexaboride.

Fuhrman W T WT   Chamorro J R JR   Alekseev P A PA   Mignot J-M JM   Keller T T   Rodriguez-Rivera J A JA   Qiu Y Y   Nikolić P P   McQueen T M TM   Broholm C L CL  

Nature communications 20180418 1


Samarium hexaboride (SmB<sub>6</sub>) is a Kondo insulator, with a narrow gap due to hybridization between localized and conduction electrons. Despite being an insulator, many samples show metal-like properties. Rare-earth purification is exceedingly difficult, and nominally pure samples may contain 2% or more of impurities. Here to determine the effects of rare-earth doping on SmB<sub>6</sub>, we synthesized and probed a series of gadolinium-doped samples. We found a relationship between specif  ...[more]

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