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Efficient metal halide perovskite light-emitting diodes with significantly improved light extraction on nanophotonic substrates.


ABSTRACT: Metal halide perovskite has emerged as a promising material for light-emitting diodes. In the past, the performance of devices has been improved mainly by optimizing the active and charge injection layers. However, the large refractive index difference among different materials limits the overall light extraction. Herein, we fabricate efficient methylammonium lead bromide light-emitting diodes on nanophotonic substrates with an optimal device external quantum efficiency of 17.5% which is around twice of the record for the planar device based on this material system. Furthermore, optical modelling shows that a high light extraction efficiency of 73.6% can be achieved as a result of a two-step light extraction process involving nanodome light couplers and nanowire optical antennas on the nanophotonic substrate. These results suggest that utilization of nanophotonic structures can be an effective approach to achieve high performance perovskite light-emitting diodes.

SUBMITTER: Zhang Q 

PROVIDER: S-EPMC6374404 | biostudies-literature | 2019 Feb

REPOSITORIES: biostudies-literature

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Efficient metal halide perovskite light-emitting diodes with significantly improved light extraction on nanophotonic substrates.

Zhang Qianpeng Q   Tavakoli Mohammad Mahdi MM   Gu Leilei L   Zhang Daquan D   Tang Lei L   Gao Yuan Y   Guo Ji J   Lin Yuanjing Y   Leung Siu-Fung SF   Poddar Swapnadeep S   Fu Yu Y   Fan Zhiyong Z  

Nature communications 20190213 1


Metal halide perovskite has emerged as a promising material for light-emitting diodes. In the past, the performance of devices has been improved mainly by optimizing the active and charge injection layers. However, the large refractive index difference among different materials limits the overall light extraction. Herein, we fabricate efficient methylammonium lead bromide light-emitting diodes on nanophotonic substrates with an optimal device external quantum efficiency of 17.5% which is around  ...[more]

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