Dataset Information

Continuously Frequency-Tuneable Plasmonic Structures for Terahertz Bio-sensing and Spectroscopy.

ABSTRACT: Plasmon-based devices are powerful for use in highly sensitive evanescent-field detection and analysis, but they exhibit the problem of limited frequency tunability for fixed structures. This feature causes problems in the multi-frequency investigations required for materials characterization, bio-related research, etc. Here, we propose and fabricate a spiral-shaped plasmonic structure that enables a continuous frequency-tuneable evanescent-field concentration in the terahertz (THz) region with simple operation. The device also increases the electric field intensity at the subwavelength aperture, thus significantly amplifying the transmission. Highly tuneable transmission bands are observed by simply rotating the spiral plasmonic structure, which are in good agreement with the behaviour expected from electromagnetic simulation. Medical examinations are performed by measuring the interactions between the frequency-tuneable plasmons and bio-samples, which enables observing distinct tissue-dependent transmission spectra and images. The developed device simultaneously offers the advantages of both plasmonic devices and frequency-tuneable devices, which can increase the availability and versatility of evanescent-field THz sensing and analysis. The mechanism presented will shed light on THz plasmonics and motivate the implementation of a variety of applications based on plasmon-mediated THz technologies.

SUBMITTER: Deng X

PROVIDER: S-EPMC6401124 | biostudies-literature | 2019 Mar

REPOSITORIES: biostudies-literature

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Continuously Frequency-Tuneable Plasmonic Structures for Terahertz Bio-sensing and Spectroscopy.

Deng Xiangying X Li Leyang L Enomoto Mitsuhiro M Kawano Yukio Y

Scientific reports 20190305 1

Plasmon-based devices are powerful for use in highly sensitive evanescent-field detection and analysis, but they exhibit the problem of limited frequency tunability for fixed structures. This feature causes problems in the multi-frequency investigations required for materials characterization, bio-related research, etc. Here, we propose and fabricate a spiral-shaped plasmonic structure that enables a continuous frequency-tuneable evanescent-field concentration in the terahertz (THz) region with ...[more]

PMID: 30837486

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Project description:Optical sensors based on surface plasmon resonance (SPR) in the attenuated total reflection (ATR) configuration in layered media have attracted considerable attention over the past decades owing to their ability of label free sensing in biomolecular interaction analysis, and highly sensitive detection of changes in refractive index and thickness, i.e. the optical thickness, of thin film adsorbates (thin film sensing). Furthermore, SPR is highly sensitive to the refractive index of the medium adjacent to the bare metal, and it allows for bulk sensing as well. When deposited at the metal/air interface, an adsorbed layer disturbs the highly localized, i.e. bound, wave at this interface and changes the plasmon resonance to allow for sensing in angular or wavelength interrogation and intensity measurement modes. A high degree of sensitivity is required for precise and efficient sensing, especially for biomolecular interaction analysis for early stage diagnostics; and besides conventional SPR (CSPR), several other configurations have been developed in recent years targeting sensitivity, including long-range SPR (LRSPR) and waveguide-coupled SPR (WGSPR) observed in MIM structures, referred here to by MIM modes, resulting from the coupling of SPRs at I/M interfaces, and Fano-type resonances occurring from broad and sharp modes coupling in layered structures. In our previous research, we demonstrated that MIM is better than CSPR for bulk sensing, and in this paper, we show that CSPR is better than MIM for thin film sensing for thicknesses of the sensing layer (SL) larger than 10 nm. We discuss and compare the sensitivity of CSPR and MIM for thin film sensing by using both experiments and theoretical calculations based on rigorous electromagnetic (EM) theory. We discuss in detail MIM modes coupling and anti-crossing, and we show that when a thin film adsorbate, i.e. a SL), is deposited on top of the outermost-layer of an optimized MIM structure, it modifies the characteristics of the coupled modes of the structure, and it reduces the electric field, both inside the SL and at the SL/air interface, and as a result, it decreases the sensitivity of the MIM versus the CSPR sensor. Our work is of critical importance to plasmonic mode coupling using MIM configurations, as well as to optical bio- and chemical-sensing.

Dataset Information

Continuously Frequency-Tuneable Plasmonic Structures for Terahertz Bio-sensing and Spectroscopy.

Publications

Continuously Frequency-Tuneable Plasmonic Structures for Terahertz Bio-sensing and Spectroscopy.

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