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Attosecond soft X-ray high harmonic generation.


ABSTRACT: High harmonic generation (HHG) of an intense laser pulse is a highly nonlinear optical phenomenon that provides the only proven source of tabletop attosecond pulses, and it is the key technology in attosecond science. Recent developments in high-intensity infrared lasers have extended HHG beyond its traditional domain of the XUV spectral range (10-150?eV) into the soft X-ray regime (150?eV to 3?keV), allowing the compactness, stability and sub-femtosecond duration of HHG to be combined with the atomic site specificity and electronic/structural sensitivity of X-ray spectroscopy. HHG in the soft X-ray spectral region has significant differences from HHG in the XUV, which necessitate new approaches to generating and characterizing attosecond pulses. Here, we examine the challenges and opportunities of soft X-ray HHG, and we use simulations to examine the optimal generating conditions for the development of high-flux, attosecond-duration pulses in the soft X-ray spectral range. This article is part of the theme issue 'Measurement of ultrafast electronic and structural dynamics with X-rays'.

SUBMITTER: Johnson AS 

PROVIDER: S-EPMC6452054 | biostudies-literature | 2019 May

REPOSITORIES: biostudies-literature

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Attosecond soft X-ray high harmonic generation.

Johnson Allan S AS   Avni Timur T   Larsen Esben W EW   Austin Dane R DR   Marangos Jon P JP  

Philosophical transactions. Series A, Mathematical, physical, and engineering sciences 20190501 2145


High harmonic generation (HHG) of an intense laser pulse is a highly nonlinear optical phenomenon that provides the only proven source of tabletop attosecond pulses, and it is the key technology in attosecond science. Recent developments in high-intensity infrared lasers have extended HHG beyond its traditional domain of the XUV spectral range (10-150 eV) into the soft X-ray regime (150 eV to 3 keV), allowing the compactness, stability and sub-femtosecond duration of HHG to be combined with the  ...[more]

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