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Gasification of coal and biomass as a net carbon-negative power source for environment-friendly electricity generation in China.

ABSTRACT: Realizing the goal of the Paris Agreement to limit global warming to 2 °C by the end of this century will most likely require deployment of carbon-negative technologies. It is particularly important that China, as the world's top carbon emitter, avoids being locked into carbon-intensive, coal-fired power-generation technologies and undertakes a smooth transition from high- to negative-carbon electricity production. We focus here on deploying a combination of coal and biomass energy to produce electricity in China using an integrated gasification cycle system combined with carbon capture and storage (CBECCS). Such a system will also reduce air pollutant emissions, thus contributing to China's near-term goal of improving air quality. We evaluate the bus-bar electricity-generation prices for CBECCS with mixing ratios of crop residues varying from 0 to 100%, as well as associated costs for carbon mitigation and cobenefits for air quality. We find that CBECCS systems employing a crop residue ratio of 35% could produce electricity with net-zero life-cycle emissions of greenhouse gases, with a levelized cost of electricity of no more than 9.2 US cents per kilowatt hour. A carbon price of approximately $52.0 per ton would make CBECCS cost-competitive with pulverized coal power plants. Therefore, our results provide critical insights for designing a CBECCS strategy in China to harness near-term air-quality cobenefits while laying the foundation for achieving negative carbon emissions in the long run.

SUBMITTER: Lu X

PROVIDER: S-EPMC6486764 | biostudies-literature | 2019 Apr

REPOSITORIES: biostudies-literature

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Gasification of coal and biomass as a net carbon-negative power source for environment-friendly electricity generation in China.

Lu Xi X Cao Liang L Wang Haikun H Peng Wei W Xing Jia J Wang Shuxiao S Cai Siyi S Shen Bo B Yang Qing Q Nielsen Chris P CP McElroy Michael B MB

Proceedings of the National Academy of Sciences of the United States of America 20190408 17

Realizing the goal of the Paris Agreement to limit global warming to 2 °C by the end of this century will most likely require deployment of carbon-negative technologies. It is particularly important that China, as the world's top carbon emitter, avoids being locked into carbon-intensive, coal-fired power-generation technologies and undertakes a smooth transition from high- to negative-carbon electricity production. We focus here on deploying a combination of coal and biomass energy to produce el ...[more]

PMID: 30962380

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Project description:Feedstocks such as coal, biomass, plastics, and their blends have the potential to serve as fuels for the thermochemical conversion process owing to their relatively high calorific values. Nevertheless, the relative proportion of these feedstock blends has a pivotal influence over the overall energy conversion efficiency. Consequently, conducting a comprehensive study to optimize the blend proportion becomes crucial in order to obtain an optimal fuel. The study aims to investigate the thermochemical characterization and kinetics of blends composed of lignite coal, southern pine biomass, and municipal waste plastic blend to optimize the blend proportion. This optimization has been achieved through an analysis of 12 distinct blends, considering factors such as combustion reaction kinetics, combustion stability, and comprehensive combustion indices. The reaction kinetics, including activation energy, pre-exponential factor, and reaction order, were estimated using various methods, including Vyazovkin, Kissinger-Akahira-Sunose, Flynn-Wall-Ozawa, Master-plot, and multidistributed activation energy methods. The investigation revealed that increasing the biomass content within the blends enhances both the combustion stability and combustion performance. The multidistributed activation energy model exhibited a good fit with both the experimental thermogravimetric and the derivative thermogravimetric curves, achieving linear regression fitness values of 0.99 and 0.95, respectively. To showcase the viability of these blends as energy generation feedstock, the optimal blend comprised of 60% biomass, 10% coal, and 30% municipal waste plastic blend, possessing the lowest activation energy (110 kJ/mol), was employed as the feedstock for the fluidized bed oxy-steam gasification process. The gasification process resulted in a synthetic gas consisting of 47.79 mol % H2, 27.96 mol % CO, 5.85 mol % CH4, and 18.38 mol % CO2 (nitrogen-free basis) with a cold gas efficiency of 72.88%. The findings of this study can offer valuable insights into global industries engaged in the thermochemical conversion of solid waste materials.

Dataset Information

Gasification of coal and biomass as a net carbon-negative power source for environment-friendly electricity generation in China.

Publications

Gasification of coal and biomass as a net carbon-negative power source for environment-friendly electricity generation in China.

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