Browse
Submit Data
Databases
API
Help

Dataset Information

0 Views

0 Connections

0 Citations

0 Reanalyses

0 Downloads

Omics score: 0

Time-resolved XUV ARPES with tunable 24-33?eV laser pulses at 30?meV resolution.

ABSTRACT: High harmonic generation of ultrafast laser pulses can be used to perform angle-resolved photoemission spectroscopy (ARPES) to map the electronic band structure of materials with femtosecond time resolution. However, currently it is difficult to reach high momenta with narrow energy resolution. Here, we combine a gas phase extreme ultraviolet (XUV) femtosecond light source, an XUV monochromator, and a time-of-flight electron analyzer to develop XUV-based time-resolved ARPES. Our technique can produce tunable photon energy between 24-33?eV with an unprecedented energy resolution of 30?meV and time resolution of 200?fs. This technique enables time-, energy- and momentum-resolved investigation of the nonequilibrium dynamics of electrons in materials with a full access to their first Brillouin zone. We evaluate the performance of this setup through exemplary measurements on various quantum materials, including WTe₂, WSe₂, TiSe₂, and Bi₂Sr₂CaCu₂O_8+?.

SUBMITTER: Sie EJ

PROVIDER: S-EPMC6684652 | biostudies-literature | 2019 Aug

REPOSITORIES: biostudies-literature

ACCESS DATA

Json Xml

Publications

Time-resolved XUV ARPES with tunable 24-33 eV laser pulses at 30 meV resolution.

Sie Edbert J EJ Rohwer Timm T Lee Changmin C Gedik Nuh N

Nature communications 20190806 1

High harmonic generation of ultrafast laser pulses can be used to perform angle-resolved photoemission spectroscopy (ARPES) to map the electronic band structure of materials with femtosecond time resolution. However, currently it is difficult to reach high momenta with narrow energy resolution. Here, we combine a gas phase extreme ultraviolet (XUV) femtosecond light source, an XUV monochromator, and a time-of-flight electron analyzer to develop XUV-based time-resolved ARPES. Our technique can pr ...[more]

PMID: 31388015

Similar Datasets

The meV XUV-RIXS facility at UE112-PGM1 of BESSY II.

Project description:Resonant inelastic X-ray scattering in the XUV-regime has been implemented at BESSY II, pushing for a few-meV bandwidth in inelastic X-ray scattering at transition metal M-edges, rare earth N-edges and the K-edges of light elements up to carbon with full polarization control. The new dedicated low-energy beamline UE112-PGM1 has been designed to provide 1 µm vertical and 20 µm horizontal beam dimensions that serve together with sub-micrometre solid-state sample positioning as the source point for a high-resolution plane grating spectrometer and a high-transmission Rowland spectrometer for rapid overview spectra. The design and commissioning results of the beamline and high-resolution spectrometer are presented. Helium autoionization spectra demonstrate a resolving power of the beamline better than 10 000 at 64 eV with a 300 lines mm-1 grating while the measured resolving power of the spectrometer in the relevant energy range is 3000 to 6000.

| S-EPMC9070711 | biostudies-literature

Single-shot spectro-temporal characterization of XUV pulses from a seeded free-electron laser.

Project description:Intense ultrashort X-ray pulses produced by modern free-electron lasers (FELs) allow one to probe biological systems, inorganic materials and molecular reaction dynamics with nanoscale spatial and femtoscale temporal resolution. These experiments require the knowledge, and possibly the control, of the spectro-temporal content of individual pulses. FELs relying on seeding have the potential to produce spatially and temporally fully coherent pulses. Here we propose and implement an interferometric method, which allows us to carry out the first complete single-shot spectro-temporal characterization of the pulses, generated by an FEL in the extreme ultraviolet spectral range. Moreover, we provide the first direct evidence of the temporal coherence of a seeded FEL working in the extreme ultraviolet spectral range and show the way to control the light generation process to produce Fourier-limited pulses. Experiments are carried out at the FERMI FEL in Trieste.

| S-EPMC4560797 | biostudies-other

Time-resolved analysis of DNA-protein interactions in living cells by UV laser pulses.

Project description:Interactions between DNA and proteins are mainly studied through chemical procedures involving bi-functional reagents, mostly formaldehyde. Chromatin immunoprecipitation is used to identify the binding between transcription factors (TFs) and chromatin, and to evaluate the occurrence and impact of histone/DNA modifications. The current bottleneck in probing DNA-protein interactions using these approaches is caused by the fact that chemical crosslinkers do not discriminate direct and indirect bindings or short-lived chromatin occupancy. Here, we describe a novel application of UV laser-induced (L-) crosslinking and demonstrate that a combination of chemical and L-crosslinking is able to distinguish between direct and indirect DNA-protein interactions in a small number of living cells. The spatial and temporal dynamics of TF bindings to chromatin and their role in gene expression regulation may thus be assessed. The combination of chemical and L-crosslinking offers an exciting and unprecedented tool for biomedical applications.

| S-EPMC5601431 | biostudies-literature

Dissociation dynamics of the diamondoid adamantane upon photoionization by XUV femtosecond pulses.

Project description:This work presents a photodissociation study of the diamondoid adamantane using extreme ultraviolet femtosecond pulses. The fragmentation dynamics of the dication is unraveled by the use of advanced ion and electron spectroscopy giving access to the dissociation channels as well as their energetics. To get insight into the fragmentation dynamics, we use a theoretical approach combining potential energy surface determination, statistical fragmentation methods and molecular dynamics simulations. We demonstrate that the dissociation dynamics of adamantane dications takes place in a two-step process: barrierless cage opening followed by Coulomb repulsion-driven fragmentation.

| S-EPMC7031298 | biostudies-literature

Nonlinear XUV signal generation probed by transient grating spectroscopy with attosecond pulses.

Project description:Nonlinear spectroscopies are utilized extensively for selective measurements of chemical dynamics in the optical, infrared, and radio-frequency regimes. The development of these techniques for extreme ultraviolet (XUV) light sources facilitates measurements of electronic dynamics on attosecond timescales. Here, we elucidate the temporal dynamics of nonlinear signal generation by utilizing a transient grating scheme with a subfemtosecond XUV pulse train and two few-cycle near-infrared pulses in atomic helium. Simultaneous detection of multiple diffraction orders reveals delays of ≥1.5 fs in higher-order XUV signal generation, which are reproduced theoretically by solving the coupled Maxwell-Schrödinger equations and with a phase grating model. The delays result in measurable order-dependent differences in the energies of transient light induced states. As nonlinear methods are extended into the attosecond regime, the observed higher-order signal generation delays will significantly impact and aid temporal and spectral measurements of dynamic processes.

| S-EPMC6437156 | biostudies-literature

Tunable Picosecond Laser Pulses via the Contrast of Two Reverse Saturable Absorption Phases in a Waveguide Platform.

Project description:How to enhance the optical nonlinearity of saturable absorption materials is an important question to improve the functionality of various applications ranging from the high power laser to photonic computational devices. We demonstrate the saturable absorption (SA) of VO2 film attributed to the large difference of optical nonlinearities between the two states of the phase-transition materials (VO2). Such VO2 film demonstrated significantly improved performance with saturation intensity higher than other existing ultrathin saturable absorbers by 3 orders due to its unique nonlinear optical mechanisms in the ultrafast phase change process. Owing to this feature, a Q-switched pulsed laser was fabricated in a waveguide platform, which is the first time to achieve picosecond pulse duration and maintain high peak power. Furthermore, the emission of this VO2 waveguide laser can be flexibly switched between the continuous-wave (CW) and pulsed operation regimes by tuning the temperature of the VO2 film, which enables VO2-based miniature laser devices with unique and versatile functions.

| S-EPMC5181842 | biostudies-literature

Tunable nanometer electrode gaps by MeV ion irradiation.

Project description:We report the use of MeV ion-irradiation-induced plastic deformation of amorphous materials to fabricate electrodes with nanometer-sized gaps. Plastic deformation of the amorphous metal Pd(80)Si(20) is induced by 4.64 MeV O(2+) ion irradiation, allowing the complete closing of a sub-micrometer gap. We measure the evolving gap size in situ by monitoring the field emission current-voltage (I-V) characteristics between electrodes. The I-V behavior is consistent with Fowler-Nordheim tunneling. We show that using feedback control on this signal permits gap size fabrication with atomic-scale precision. We expect this approach to nanogap fabrication will enable the practical realization of single molecule controlled devices and sensors.

| S-EPMC3338580 | biostudies-other

Tunable Broadband Nonlinear Optical Properties of Black Phosphorus Quantum Dots for Femtosecond Laser Pulses.

Project description:Broadband nonlinear optical properties from 500 to 1550 nm of ultrasmall black phosphorus quantum dots (BPQDs) have been extensively investigated by using the open-aperture Z-scan technique. Our results show that BPQDs exhibit significant nonlinear absorption in the visible range, but saturable absorption in the near-infrared range under femtosecond excitation. The calculated nonlinear absorption coefficients were found to be (7.49 ± 0.23) × 10-3, (1.68 ± 0.078) × 10-3 and (0.81 ± 0.03) × 10-3 cm/GW for 500, 700 and 900 nm, respectively. Femtosecond pump-probe measurements performed on BPQDs revealed that two-photon absorption is responsible for the observed nonlinear absorption. The saturable absorption behaviors observed at 1050, 1350 and 1550 nm are due to ground-state bleaching induced by photo-excitation. Our results suggest that BPQDs have great potential in applications as broadband optical limiters in the visible range or saturable absorbers in the near-infrared range for ultrafast laser pulses. These ultrasmall BPQDs are potentially useful as broadband optical elements in ultrafast photonics devices.

| S-EPMC5459120 | biostudies-other

Single Shot Polarization Characterization of XUV FEL Pulses from Crossed Polarized Undulators.

Project description:Polarization control is a key feature of light generated by short-wavelength free-electron lasers. In this work, we report the first experimental characterization of the polarization properties of an extreme ultraviolet high gain free-electron laser operated with crossed polarized undulators. We investigate the average degree of polarization and the shot-to-shot stability and we analyze aspects such as existing possibilities for controlling and switching the polarization state of the emitted light. The results are in agreement with predictions based on Gaussian beams propagation.

| S-EPMC4551986 | biostudies-other

Time-resolved plasmon-assisted generation of optical-vortex pulses.

Project description:The microscopic mechanism of the light-matter interactions that induce orbital angular momentum (OAM) in electromagnetic fields is not thoroughly understood. In this work, we employ Archimedean spiral vortex generators in time-resolved numerical simulations using the Octopus code to observe the behind-the-scenes of OAM generation. We send a perfect circularly-polarized plane-wave light onto plasmonic optical vortex generators and observe the resulting twisted light formation with complete spatio-temporal information. In agreement with previous works, we find that emission from the plasmonic spiral branches shapes the vortex-like structure and governs the OAM generation in the outgoing electromagnetic field. To characterize the generated beam further, we emulate the emission from vortex generators with current emitters preserving the spiral geometry. We subject a point-particle system to the generated field and record the orbital angular momentum transfer between the electromagnetic field and the point particle. Finally, we probe the OAM density locally by studying the induced classical trajectory of point particles, which provides further insight into the spatio-temporal features of the induced OAM.

| S-EPMC10484912 | biostudies-literature

OmicsDI is part of the ELIXIR infrastructure

OmicsDI is an Elixir interoperability service. Learn more ›

Tweets

OmicsDI Databases

PRIDE
PeptideAtlas
MassIVE
JPOST Repository
Physiome Model Repository

EGA
EVA
ENA
LINCS
PAXDB
Cell Collective

MetaboLights
Metabolomics Workbench
MetabolomeExpress
GNPS
BioModels
FAIRDOMHub

ArrayExpress
dbGaP
ExpressionAtlas
GEO
NODE

Information

Databases
Help
API
Contact us
Code on GitHub
Terms of use
Submit Data