Dataset Information

Ricocheting Droplets Moving on Super-Repellent Surfaces.

ABSTRACT: Droplet bouncing on repellent solid surfaces (e.g., the lotus leaf effect) is a common phenomenon that has aroused interest in various fields. However, the scenario of a droplet bouncing off another droplet (either identical or distinct chemical composition) while moving on a solid material (i.e., ricocheting droplets, droplet billiards) is scarcely investigated, despite it having fundamental implications in applications including self-cleaning, fluid transport, and heat and mass transfer. Here, the dynamics of bouncing collisions between liquid droplets are investigated using a friction-free platform that ensures ultrahigh locomotion for a wide range of probing liquids. A general prediction on bouncing droplet-droplet contact time is elucidated and bouncing droplet-droplet collision is demonstrated to be an extreme case of droplet bouncing on surfaces. Moreover, the maximum deformation and contact time are highly dependent on the position where the collision occurs (i.e., head-on or off-center collisions), which can now be predicted using parameters (i.e., effective velocity, effective diameter) through the concept of an effective interaction region. The results have potential applications in fields ranging from microfluidics to repellent coatings.

SUBMITTER: Pan S

PROVIDER: S-EPMC6839626 | biostudies-literature | 2019 Nov

REPOSITORIES: biostudies-literature

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Publications

Ricocheting Droplets Moving on Super-Repellent Surfaces.

Pan Shuaijun S Guo Rui R Richardson Joseph J JJ Berry Joseph D JD Besford Quinn A QA Björnmalm Mattias M Yun Gyeongwon G Wu Ruoxi R Lin Zhixing Z Zhong Qi-Zhi QZ Zhou Jiajing J Sun Qiang Q Li Jianhua J Lu Yanbing Y Dong Zhichao Z Banks Margaret Katherine MK Xu Weijian W Jiang Jianhui J Jiang Lei L Caruso Frank F

Advanced science (Weinheim, Baden-Wurttemberg, Germany) 20190912 21

Droplet bouncing on repellent solid surfaces (e.g., the lotus leaf effect) is a common phenomenon that has aroused interest in various fields. However, the scenario of a droplet bouncing off another droplet (either identical or distinct chemical composition) while moving on a solid material (i.e., ricocheting droplets, droplet billiards) is scarcely investigated, despite it having fundamental implications in applications including self-cleaning, fluid transport, and heat and mass transfer. Here, ...[more]

PMID: 31728297

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Project description:Wetting plays a major role in the close interactions between liquids and solid surfaces, which can be tailored by modifying the chemistry as well as the structures of the surfaces' outermost layer. Several methodologies, such as chemical vapor deposition, physical vapor deposition, electroplating, and chemical reactions, among others, have been adopted for the alteration/modification of such interactions suitable for various applications. However, the fabrication of low-contact line-pinning hydrophobic surfaces via simple and easy methods remains an open challenge. In this work, we exploit one-step and multiple-step silicone oil (5-100 cSt) grafting on smooth silicon substrates (although the technique is suitable for other substrates), looking closely at the effect of viscosity as well as the volume and layers (one to five) of oil grafted as a function of the deposition method. Remarkably, the optimization of grafting of silicone oil fabrication results in non-wetting surfaces with extremely low contact angle hysteresis (CAH) below 1° and high contact angles (CAs) of ∼108° after a single grafting step, which is an order of magnitude smaller than the reported values of previous works on silicone oil-grafted surfaces. Moreover, the different droplet-surface interactions and pinning behavior can additionally be tailored to the specific application with CAH ranging from 1 to 20° and sliding angles between 1.5 and 60° (for droplet volumes of 3 μL), depending on the fabrication parameters adopted. In terms of roughness, all the samples (independent of the grafting parameters) showed small changes in the root-mean-square roughness below 20 nm. Lastly, stability analysis of the grafting method reported here under various conditions shows that the coating is quite stable under mechanical vibrations (bath ultrasonication) and in a chemical environment (ultrasonication in a bath of ethanol) but loses its low-pinning characteristics when exposed to saturated steam at T ∼ 99 °C. The findings presented here provide a basis for selecting the most appropriate and suitable method and parameters for silicone oil grafting aimed at low pinning and low hysteresis surfaces for specific applications.

Dataset Information

Ricocheting Droplets Moving on Super-Repellent Surfaces.

Publications

Ricocheting Droplets Moving on Super-Repellent Surfaces.

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