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Complex multiphase organohydrogels with programmable mechanics toward adaptive soft-matter machines.


ABSTRACT: Many biological organisms can tune their mechanical properties to adapt to environments in multistable modes, but the current synthetic materials, with bistable states, have a limited ability to alter mechanical stiffness. Here, we constructed programmable organohydrogels with multistable mechanical states by an on-demand modular assembly of noneutectic phase transition components inside microrganogel inclusions. The resultant multiphase organohydrogel exhibits precisely controllable thermo-induced stepwise switching (i.e., triple, quadruple, and quintuple switching) mechanics and a self-healing property. The organohydrogel was introduced into the design of soft-matter machines, yielding a soft gripper with adaptive grasping through stiffness matching with various objects under pneumatic-thermal hybrid actuation. Meanwhile, a programmable adhesion of octopus-inspired robotic tentacles on a wide range of surface morphologies was realized. These results demonstrated the applicability of these organohydrogels in lifelike soft robotics in unconstructed and human body environments.

SUBMITTER: Zhuo S 

PROVIDER: S-EPMC6994219 | biostudies-literature | 2020 Jan

REPOSITORIES: biostudies-literature

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Complex multiphase organohydrogels with programmable mechanics toward adaptive soft-matter machines.

Zhuo Shuyun S   Zhao Ziguang Z   Xie Zhexin Z   Hao Yufei Y   Xu Yichao Y   Zhao Tianyi T   Li Huanjun H   Knubben Elias M EM   Wen Li L   Jiang Lei L   Liu Mingjie M  

Science advances 20200131 5


Many biological organisms can tune their mechanical properties to adapt to environments in multistable modes, but the current synthetic materials, with bistable states, have a limited ability to alter mechanical stiffness. Here, we constructed programmable organohydrogels with multistable mechanical states by an on-demand modular assembly of noneutectic phase transition components inside microrganogel inclusions. The resultant multiphase organohydrogel exhibits precisely controllable thermo-indu  ...[more]

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