Dataset Information

Source contribution analysis of mercury deposition using an enhanced CALPUFF-Hg in the central Pearl River Delta, China.

ABSTRACT: Atmospheric mercury (Hg) poses human health and ecological risks once deposited and bio-accumulated through food chains. Source contribution analysis of Hg deposition is essential to formulating emission control strategies to alleviate the adverse impact of Hg release from anthropogenic sources. In this study, a Hg version of California Puff Dispersion Modeling (denoted as CALPUFF-Hg) system with added Hg environmental processes was implemented to simulate the Hg concentration and deposition in the central region of the Pearl River Delta (cPRD) at 1?km?×?1?km resolution. The contributions of eight source sectors to Hg deposition were evaluated. Model results indicated that the emission from cement production was the largest contributor to Hg deposition, accounting for 13.0%, followed by coal-fired power plants (6.5%), non-ferrous metal smelting (5.4%), iron and steel production (3.5%), and municipal solid waste incineration (3.4%). The point sources that released a higher fraction of gaseous oxidized mercury, such as cement production and municipal solid waste incineration, were the most significant contributors to local deposition. In this intensive industrialized region, large point sources contributed 67-94% of total Hg deposition of 6 receptors which were the nearest grid-cells from top five Hg emitters of the domain and the largest municipal solid waste incinerator in Guangzhou. Based on the source apportionment results, cement production and the rapidly growing municipal solid waste incineration are identified as priority sectors for Hg emission control in the cPRD region.

SUBMITTER: Xu H

PROVIDER: S-EPMC7654097 | biostudies-literature | 2019 Jul

REPOSITORIES: biostudies-literature

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Source contribution analysis of mercury deposition using an enhanced CALPUFF-Hg in the central Pearl River Delta, China.

Xu Hui H Zhu Yun Y Wang Long L Lin Che-Jen CJ Jang Carey C Zhou Qin Q Yu Bin B Wang Shuxiao S Xing Jia J Yu Lian L

Environmental pollution (Barking, Essex : 1987) 20190406

Atmospheric mercury (Hg) poses human health and ecological risks once deposited and bio-accumulated through food chains. Source contribution analysis of Hg deposition is essential to formulating emission control strategies to alleviate the adverse impact of Hg release from anthropogenic sources. In this study, a Hg version of California Puff Dispersion Modeling (denoted as CALPUFF-Hg) system with added Hg environmental processes was implemented to simulate the Hg concentration and deposition in ...[more]

PMID: 31085469

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Project description:Pb and Cd accumulation in riparian soils and river sediments in river basins is a challenging pollution issue due to the persistence and bioaccumulation of these two trace metals. Understanding the migration characteristics and input sources of these metals is the key to preventing metal pollution. This study was conducted to explore the contents, geochemical fractionation, and input sources of Pb and Cd in riparian soils and river sediments from three lower reaches of the Pearl River Delta located in the Guangdong-Hong Kong-Macao Greater Bay Area. The total concentration of all Pb and Cd values exceeded the background values to varying degrees, and the exchangeable fraction of Cd in riparian soils and river sediments accounted for the largest proportion, while that of Pb was dominated by the residual fraction. Geoaccumulation index calculations showed that in the riparian soils, the average accumulation degree of Pb (0.52) in the Beijiang River (BJR) was the highest, while that of Cd (2.04) in the Xijiang River (XJR) was the highest. Unlike that in riparian soils, the maximum accumulation of Pb (0.76) and Cd (3.01) in river sediments both occurred in the BJR. Furthermore, the enrichment factor results also showed that Pb and Cd in the riparian soils and river sediments along the BJR were higher than those in the XJR and Dongjiang River (DJR). The relationship between enrichment factors and nonresidual fractions further proved that the enrichment factors of Cd were significantly correlated with the nonresidual fractions of Cd, which may imply various anthropogenic sources of Cd in the three reaches. Moreover, source identification based on principal component analysis (PCA) and Pb isotope ratio analysis indicated that riparian soils and river sediments have inconsistent pollution source structures. The PCA results showed that Pb and Cd were homologous inputs in the DJR, and there were significant differences only in the riparian soils and river sediments. Pb isotope tracing results further showed that the bedrock of high geological background from upstream may be the main reason for Cd accumulation in the XJR. However, the ultrahigh accumulation of Cd in the BJR is mainly caused by the input of the upstream mining and metallurgy industry. The control of upstream input sources will be the key to the prevention of trace metal pollution in these regions.

Project description:BackgroundIn recent years, frequent outbreaks of dengue fever (DF) have become an increasingly serious public health issue in China, especially in the Pearl River Delta (PRD) with fast socioeconomic developments. Previous studies mainly focused on the historic DF epidemics, their influencing factors, and the prediction of DF risks. However, the future risks of this disease under both different socioeconomic development and representative concentration pathways (RCPs) scenarios remain little understood.Methodology and principal findingsIn this study, a spatial dataset of gross domestic product (GDP), population density, and land use and land coverage (LULC) in 2050 and 2070 was obtained by simulation based on the different shared socioeconomic pathways (SSPs), and the future climatic data derived from the RCP scenarios were integrated into the Maxent models for predicting the future DF risk in the PRD region. Among all the variables included in this study, socioeconomics factors made the dominant contribution (83% or so) during simulating the current spatial distribution of the DF epidemics in the PRD region. Moreover, the spatial distribution of future DF risk identified by the climatic and socioeconomic (C&S) variables models was more detailed than that of the climatic variables models. Along with global warming and socioeconomic development, the zones with DF high and moderate risk will continue to increase, and the population at high and moderate risk will reach a maximum of 48.47 million (i.e., 63.78% of the whole PRD) under the RCP 4.5/SSP2 in 2070.ConclusionsThe increasing DF risk may be an inevitable public health threat in the PRD region with rapid socioeconomic developments and global warming in the future. Our results suggest that curbs in emissions and more sustainable socioeconomic growth targets offer hope for limiting the future impact of dengue, and effective prevention and control need to continue to be strengthened at the junction of Guangzhou-Foshan, north-central Zhongshan city, and central-western Dongguan city. Our study provides useful clues for relevant hygienic authorities making targeted adapting strategies for this disease.

Dataset Information

Source contribution analysis of mercury deposition using an enhanced CALPUFF-Hg in the central Pearl River Delta, China.

Publications

Source contribution analysis of mercury deposition using an enhanced CALPUFF-Hg in the central Pearl River Delta, China.

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