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Twist-angle dependence of moire excitons in WS2/MoSe2 heterobilayers.


ABSTRACT: Moiré lattices formed in twisted van der Waals bilayers provide a unique, tunable platform to realize coupled electron or exciton lattices unavailable before. While twist angle between the bilayer has been shown to be a critical parameter in engineering the moiré potential and enabling novel phenomena in electronic moiré systems, a systematic experimental study as a function of twist angle is still missing. Here we show that not only are moiré excitons robust in bilayers of even large twist angles, but also properties of the moiré excitons are dependant on, and controllable by, the moiré reciprocal lattice period via twist-angle tuning. From the twist-angle dependence, we furthermore obtain the effective mass of the interlayer excitons and the electron inter-layer tunneling strength, which are difficult to measure experimentally otherwise. These findings pave the way for understanding and engineering rich moiré-lattice induced phenomena in angle-twisted semiconductor van der Waals heterostructures.

SUBMITTER: Zhang L 

PROVIDER: S-EPMC7675978 | biostudies-literature | 2020 Nov

REPOSITORIES: biostudies-literature

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Twist-angle dependence of moiré excitons in WS<sub>2</sub>/MoSe<sub>2</sub> heterobilayers.

Zhang Long L   Zhang Zhe Z   Wu Fengcheng F   Wang Danqing D   Gogna Rahul R   Hou Shaocong S   Watanabe Kenji K   Taniguchi Takashi T   Kulkarni Krishnamurthy K   Kuo Thomas T   Forrest Stephen R SR   Deng Hui H  

Nature communications 20201118 1


Moiré lattices formed in twisted van der Waals bilayers provide a unique, tunable platform to realize coupled electron or exciton lattices unavailable before. While twist angle between the bilayer has been shown to be a critical parameter in engineering the moiré potential and enabling novel phenomena in electronic moiré systems, a systematic experimental study as a function of twist angle is still missing. Here we show that not only are moiré excitons robust in bilayers of even large twist angl  ...[more]

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