Dataset Information

Sustainable Biocomposites from Recycled Bale Wrap Plastic and Agave Fiber: Processing and Property Evaluation.

ABSTRACT: Plastic recycling to make sustainable materials is considered one of the biggest initiatives toward a greener environment and socioeconomic development. This research aims to investigate the properties of a blend of recycled bale wrap linear low-density polyethylene (rLLDPE) and polypropylene (PP) (rLLDPE/PP 50:50 wt % matrix), which was further reinforced with 25 wt % agave fiber prepared by injection-molding. Different ratios of a combined industrial compatibilizer (maleic anhydride-grafted PP/PE) were used (1-3 wt %), which were compared with a synthesized compatibilizer made from maleic anhydride-PP/rLLDPE in terms of mechanical and thermomechanical properties of the biocomposites. Incorporation of the compatibilizer in the composite improved the interfacial adhesion between the hydrophobic matrix and the hydrophilic agave fiber, which further increased the mechanical properties and heat deflection temperature of the composite. Scanning electron microscopy showed enhanced compatibility and adhesion between the fiber and the matrix by inclusion of 2 wt % compatibilizer. The synthesized compatibilizer-blended composite showed better mechanical properties than the industrial one, which indicates the potential application of this composite (around 62% recycled material) in the manufacture of packaging materials and commodity products.

SUBMITTER: Chowdhury IH

PROVIDER: S-EPMC7860101 | biostudies-literature | 2021 Feb

REPOSITORIES: biostudies-literature

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Sustainable Biocomposites from Recycled Bale Wrap Plastic and Agave Fiber: Processing and Property Evaluation.

Chowdhury Iftekhar H IH Abdelwahab Mohamed A MA Misra Manjusri M Mohanty Amar K AK

ACS omega 20210119 4

Plastic recycling to make sustainable materials is considered one of the biggest initiatives toward a greener environment and socioeconomic development. This research aims to investigate the properties of a blend of recycled bale wrap linear low-density polyethylene (rLLDPE) and polypropylene (PP) (rLLDPE/PP 50:50 wt % matrix), which was further reinforced with 25 wt % agave fiber prepared by injection-molding. Different ratios of a combined industrial compatibilizer (maleic anhydride-grafted PP ...[more]

PMID: 33553903

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Project description:Carbon fiber reinforced composites have exceptional potential to play a key role in the materials world of our future. However, their success undoubtedly depends on the extent they can contribute to advance a global sustainability objective. Utilizing polymers in these composites that can be potentially derived from biomasses would be certainly vital for next-generation manufacturing practices. Nevertheless, deep understanding and tailoring fiber-matrix interactions are crucial issues in order to design carbon fiber reinforced sustainable resource-based biocomposites. In this study, cellulose derivatives (cellulose propionate and cellulose acetate butyrate) are utilized as model polymer matrices that can be potentially fabricated from biomasses, and the mechanical properties of the prepared short carbon fiber reinforced composites are engineered by means of a functional biobased lignin coating on the fiber surface. Furthermore, polyamide 6 based composites are also prepared, the monomer of this polymer could be obtained using C6 sugars derived from lignocellulosic biomasses in the future (through 5-hydroxymethylfurfural). Lignin was successfully immobilized on the carbon fiber surface via an industrially scalable benign epoxidation reaction. The surface modification had a beneficial impact on the mechanical properties of cellulose propionate and polyamide 6 composites. Furthermore, our results also revealed that cellulose-based matrices are highly sensitive to the presence of rigid fiber segments that restrict polymer chain movements and facilitate stress development. It follows that the physicochemical properties of the cellulosic matrices (molecular weight, crystallinity), associated with polymer chain mobility, might need to be carefully considered when designing these composites. At the same time, polyamide 6 showed excellent ability to accommodate short carbon fibers without leading to a largely brittle material, in this case, a maximum tensile strength of ~136 MPa was obtained at 20 wt% fiber loading. These results were further contrasted with that of a petroleum-based polypropylene matrix exhibiting inferior mechanical properties. Our study clearly indicates that carbon fiber reinforced polymers derived and designed using biomass-derived resources can be promising green materials for a sustainable future.

Dataset Information

Sustainable Biocomposites from Recycled Bale Wrap Plastic and Agave Fiber: Processing and Property Evaluation.

Publications

Sustainable Biocomposites from Recycled Bale Wrap Plastic and Agave Fiber: Processing and Property Evaluation.

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