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Ultrafast non-excitonic valley Hall effect in MoS₂/WTe₂ heterobilayers.

ABSTRACT: The valley Hall effect (VHE) in two-dimensional (2D) van der Waals (vdW) crystals is a promising approach to study the valley pseudospin. Most experiments so far have used bound electron-hole pairs (excitons) through local photoexcitation. However, the valley depolarization of such excitons is fast, so that several challenges remain to be resolved. We address this issue by exploiting a unipolar VHE using a heterobilayer made of monolayer MoS₂/WTe₂ to exhibit a long valley-polarized lifetime due to the absence of electron-hole exchange interaction. The unipolar VHE is manifested by reduced photoluminescence at the MoS₂ A exciton energy. Furthermore, we provide quantitative information on the time-dependent valley Hall dynamics by performing the spatially-resolved ultrafast Kerr-rotation microscopy; we find that the valley-polarized electrons persist for more than 4 nanoseconds and the valley Hall mobility exceeds 4.49 × 10³ cm²/Vs, which is orders of magnitude larger than previous reports.

SUBMITTER: Lee J

PROVIDER: S-EPMC7955044 | biostudies-literature |

REPOSITORIES: biostudies-literature

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