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Observation of monochromatic and coherent luminescence from nanocavities of GaN nanowall network.

ABSTRACT: Scaling-down the size of semiconductor cavity lasers and engineering their electromagnetic environment in the Purcell regime can bring about spectacular advance in nanodevices fabrication. We report here an unprecedented observation of a coherent Cathodoluminescence from GaN nanocavities (20-100 nm). Incident lower energy (< 15 kV) electron beams excite the band edge UV emission from the walls of the network whereas for higher energies, the emitted photons are spontaneously down converted into NIR and preferentially emerge from the nanocavities. Non-centrosymmetric structure of GaN and its nanowall geometry together facilitate this unique observation which is substantiated by our numerical results. At cryogenic temperatures, an intense and narrow laser-like NIR beam emanates out of the nanocavities. The work promises the possibility of fabrication of very high density (over 10⁸/cm²) cavity lasers that are addressable by simple deflection and tuning of incident electron beams.

SUBMITTER: Shamoon D

PROVIDER: S-EPMC8087758 | biostudies-literature |

REPOSITORIES: biostudies-literature

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Project description:The intensive measures of luminescence in a GaN/InGaN multiple quantum well system are used to examine the thermodynamics and phenomenological structure. The radiative /nonradiative transitions along with absorbed or emitted phonons that occur between the different quantum states of the electrons and holes associated with these processes make the quantum efficiency of a semiconductor nanosystem in an equilibrium state an extensive property. It has long been recognized that tuning of the indium (In) composition in InGaN interlayers gives the potential to obtain a spectrum in the near-infrared to near-ultraviolet spectral range. The thermodynamic intensive properties, including the Debye temperature, carrier temperature, and junction temperature, are the most appropriate metrics to describe the optical-related interactions inherent in a given heterostructure and so can be used as the state variables for understanding the quantum exchange behaviors. The energetic features of the quantum processes are characterized based on analysis of the intensive parameters as determined by means of electroluminescence (EL) and photoluminescence (PL) spectroscopy and current-voltage measurement and then correlated with the designed InGaN/GaN microstructures. According to the McCumber-Sturge theory, the EL and PL Debye temperatures obtained experimentally signal the strength of the electron-phonon and photon-phonon interaction, respectively, while the EL and PL carrier/junction temperatures correspond to the carrier localization. Higher EL Debye temperatures and lower EL carrier/junction temperatures reflect significantly higher luminescence quantum yields, indicative of electron-phonon coupling in the transfer of thermal energy between the confined electrons and the enhancement by excited phonons of heat-assisted emissions. On the other hand, the observation of low luminescence efficiency, corresponding to the lower PL Debye temperatures and higher PL carrier/junction temperatures, is attributed to photon-phonon coupling. These findings are in good accordance to the dependence of the EL and PL quantum efficiency on the In-content of the InGaN/GaN barriers, suggesting that the characteristic Debye and carrier/junction temperatures are intensive parameters useful for assessing the optical properties of a nano-engineered semiconductor heterostructure.

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Observation of monochromatic and coherent luminescence from nanocavities of GaN nanowall network.

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