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In Situ Electric-Induced Switchable Transparency and Wettability on Laser-Ablated Bioinspired Paraffin-Impregnated Slippery Surfaces.

ABSTRACT: Switchable wetting and optical properties on a surface is synergistically realized by mechanical or temperature stimulus. Unfortunately, in situ controllable wettability together with programmable transparency on 2D/3D surfaces is rarely explored. Herein, Joule-heat-responsive paraffin-impregnated slippery surface (JR-PISS) is reported by the incorporation of lubricant paraffin, superhydrophobic micropillar-arrayed elastomeric membrane, and embedded transparent silver nanowire thin-film heater. Owing to its good flexibility, in situ controllable locomotion for diverse liquids on planar/curved JR-PISS is unfolded by alternately applying/discharging low electric-trigger of 6 V. Simultaneously, optical visibility can be reversibly converted between opaque and transparent modes. The switching principle is that in the presence of Joule-heat, solid paraffin would be melt and swell within 20 s to enable a slippery surface for decreasing light scattering and frictional force derived from contact angle hysteresis (F_CAH ). Once Joule-heat is discharged, undulating rough surface would reconfigure by cold-shrinkage of paraffin within 8 s to render light blockage and high F_CAH . Upon its portable merit, in situ thermal management, programmable visibility, as well as steering functionalized droplets by electric-activated JR-PISSs are successfully deployed. Compared with previous Nepenthes-inspired slippery surfaces, the current JR-PISS is more competent for in situ harnessing optical and wetting properties on-demand.

SUBMITTER: Chen C

PROVIDER: S-EPMC8292917 | biostudies-literature |

REPOSITORIES: biostudies-literature

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Project description:Young's equation is fundamental to the concept of the wettability of a solid surface. It defines the contact angle for a droplet on a solid surface through a local equilibrium at the three-phase contact line. Recently, the concept of a liquid Young's law contact angle has been developed to describe the wettability of slippery liquid-infused porous surfaces (SLIPS) by droplets of an immiscible liquid. In this work, we present a new method to fabricate biphilic SLIP surfaces and show how the wettability of the composite SLIPS can be exploited with a macroscopic wedge-shaped pattern of two distinct lubricant liquids. In particular, we report the development of composite liquid surfaces on silicon substrates based on lithographically patterning a Teflon AF1600 coating and a superhydrophobic coating (Glaco Mirror Coat Zero), where the latter selectively dewets from the former. This creates a patterned base surface with preferential wetting to matched liquids: the fluoropolymer PTFE with a perfluorinated oil Krytox and the hydrophobic silica-based GLACO with olive oil (or other mineral oils or silicone oil). This allows us to successively imbibe our patterned solid substrates with two distinct oils and produce a composite liquid lubricant surface with the oils segregated as thin films into separate domains defined by the patterning. We illustrate that macroscopic wedge-shaped patterned SLIP surfaces enable low-friction droplet self-propulsion. Finally, we formulate an analytical model that captures the dependence of the droplet motion as a function of the wettability of the two liquid lubricant domains and the opening angle of the wedge. This allows us to derive scaling relationships between various physical and geometrical parameters. This work introduces a new approach to creating patterned liquid lubricant surfaces, demonstrates long-distance droplet self-propulsion on such surfaces, and sheds light on the interactions between liquid droplets and liquid surfaces.

Dataset Information

In Situ Electric-Induced Switchable Transparency and Wettability on Laser-Ablated Bioinspired Paraffin-Impregnated Slippery Surfaces.

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