Dataset Information

Atmospheric observations suggest methane emissions in north-eastern China growing with natural gas use.

ABSTRACT: The dramatic increase of natural gas use in China, as a substitute for coal, helps to reduce CO₂ emissions and air pollution, but the climate mitigation benefit can be offset by methane leakage into the atmosphere. We estimate methane emissions from 2010 to 2018 in four regions of China using the GOSAT satellite data and in-situ observations with a high-resolution (0.1° × 0.1°) inverse model and analyze interannual changes of emissions by source sectors. We find that estimated methane emission over the north-eastern China region contributes the largest part (0.77 Tg CH₄ yr^-1) of the methane emission growth rate of China (0.87 Tg CH₄ yr^-1) and is largely attributable to the growth in natural gas use. The results provide evidence of a detectable impact on atmospheric methane observations by the increasing natural gas use in China and call for methane emission reductions throughout the gas supply chain and promotion of low emission end-use facilities.

SUBMITTER: Wang F

PROVIDER: S-EPMC9672054 | biostudies-literature | 2022 Nov

REPOSITORIES: biostudies-literature

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Atmospheric observations suggest methane emissions in north-eastern China growing with natural gas use.

Wang Fenjuan F Maksyutov Shamil S Janardanan Rajesh R Tsuruta Aki A Ito Akihiko A Morino Isamu I Yoshida Yukio Y Tohjima Yasunori Y Kaiser Johannes W JW Lan Xin X Zhang Yong Y Mammarella Ivan I Lavric Jost V JV Matsunaga Tsuneo T

Scientific reports 20221117 1

The dramatic increase of natural gas use in China, as a substitute for coal, helps to reduce CO<sub>2</sub> emissions and air pollution, but the climate mitigation benefit can be offset by methane leakage into the atmosphere. We estimate methane emissions from 2010 to 2018 in four regions of China using the GOSAT satellite data and in-situ observations with a high-resolution (0.1° × 0.1°) inverse model and analyze interannual changes of emissions by source sectors. We find that estimated methane ...[more]

PMID: 36396723

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Project description:Understanding emissions of methane from legacy and ongoing shale gas development requires both regional studies that assess the frequency of emissions and case studies that assess causation. We present the first direct measurements of emissions in a case study of a putatively leaking gas well in the largest shale gas play in the United States. We quantify atmospheric methane emissions in farmland >2 km from the nearest shale gas well cited for casing and cementing issues. We find that emissions are highly heterogeneous as they travel long distances in the subsurface. Emissions were measured near observed patches of dead vegetation and methane bubbling from a stream. An eddy covariance flux tower, chamber flux measurements, and a survey of enhancements of the near-surface methane mole fraction were used to quantify emissions and evaluate the spatial and temporal variability. We combined eddy covariance measurements with the survey of the methane mole fraction to estimate total emissions over the study area (2,800 m2). Estimated at ∼6 kg CH4 day-1, emissions were spatially heterogeneous but showed no temporal trends over 6 months. The isotopic signature of the atmospheric CH4 source (δ13CH4) was equal to -29‰, consistent with methane of thermogenic origin and similar to the isotopic signature of the gas reported from the nearest shale gas well. While the magnitude of emissions from the potential leak is modest compared to large emitters identified among shale gas production sites, it is large compared to estimates of emissions from single abandoned wells. Since other areas of emissions have been identified close to this putatively leaking well, our estimate of emissions likely represents only a portion of total emissions from this event. More comprehensive quantification will require more extensive spatial and temporal sampling of the locations of gas migration to the surface as well as an investigation into the mechanisms of subsurface gas migration. This work highlights an example of atmospheric methane emissions from potential stray gas migration at a location far from a well pad, and further research should explore the frequency and mechanisms behind these types of events to inform careful and strategic natural gas development.

Dataset Information

Atmospheric observations suggest methane emissions in north-eastern China growing with natural gas use.

Publications

Atmospheric observations suggest methane emissions in north-eastern China growing with natural gas use.

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