Browse
Submit Data
Databases
API
Help

Dataset Information

0 Views

0 Connections

0 Citations

0 Reanalyses

0 Downloads

Omics score: 0

Faraday rotation and photoluminescence in heavily Tb(3+)-doped GeO2-B2O3-Al2O3-Ga2O3 glasses for fiber-integrated magneto-optics.

ABSTRACT: We report on the magneto-optical (MO) properties of heavily Tb(3+)-doped GeO2-B2O3-Al2O3-Ga2O3 glasses towards fiber-integrated paramagnetic MO devices. For a Tb(3+) ion concentration of up to 9.7 × 10(21) cm(-3), the reported glass exhibits an absolute negative Faraday rotation of ~120 rad/T/m at 632.8 nm. The optimum spectral ratio between Verdet constant and light transmittance over the spectral window of 400-1500 nm is found for a Tb(3+) concentration of ~6.5 × 10(21) cm(-3). For this glass, the crystallization stability, expressed as the difference between glass transition temperature and onset temperature of melt crystallization exceeds 100 K, which is a prerequisite for fiber drawing. In addition, a high activation energy of crystallization is achieved at this composition. Optical absorption occurs in the NUV and blue spectral region, accompanied by Tb(3+) photoluminescence. In the heavily doped materials, a UV/blue-to-green photo-conversion gain of ~43% is achieved. The lifetime of photoluminescence is ~2.2 ms at a stimulated emission cross-section σem of ~1.1 × 10(-21) cm(2) for ~ 5.0 × 10(21) cm(-3) Tb(3+). This results in an optical gain parameter σem*τ of ~2.5 × 10(-24) cm(2)s, what could be of interest for implementation of a Tb(3+) fiber laser.

SUBMITTER: Gao G

PROVIDER: S-EPMC4354094 | biostudies-other | 2015

REPOSITORIES: biostudies-other

ACCESS DATA

Json Xml

Similar Datasets

Magneto-optical borogermanate glasses and fibers containing Tb<sup>3</sup>.

Project description:New glass compositions containing high concentrations of Tb3+ ions were developed aiming at the production of magneto-optical (MO) fibers. This work reports on the structural and MO properties of a new glass composition based on (100 - x)(41GeO2-25B2O3-4Al2O3-10Na2O-20BaO) - xTb4O7. Morphological analysis (HR-TEM) of the sample with the highest concentration of Tb3+ ions confirmed the homogeneous distribution of Tb3+ ions and the absence of nanoclusters. All the samples presented excellent thermal stability against crystallization (ΔT > 100 °C). An optical fiber was manufactured by a fiber drawing process. The UV-Vis spectra of the glasses showed Tb3+ electronic transitions and optical windows varying from 0.4 to 1.6 μm. The magneto-optical properties and the paramagnetic behaviors of the glasses were investigated using Faraday rotation experiments. The Verdet constant (VB) values were calculated at 500, 650, 880, 1050, 1330, and 1550 nm. The maximum VB values obtained at 650 and 1550 nm for the glass with x = 18 mol% were -128 and - 17.6 rad T-1 m-1, respectively. The VB values at 500 and 1550 nm for the optical fiber containing 8 mol% of Tb4O7 were - 110.2 and - 9.5 rad T-1 m-1, respectively, while the optical loss at around 880 nm was 6.4 dB m-1.

| S-EPMC8110553 | biostudies-literature

Natural weak value amplification in Fano resonance and giant Faraday rotation in magneto-plasmonic crystal.

Project description:The extraordinary concept of weak value amplification can be formulated within the realm of wave interference as nearly destructive interference between the eigenstates of the measuring observable. Here we report on a phenomenon of interferometric weak value amplification of small polarization rotation in Fano resonance that evolves completely naturally due to near destructive spectral domain interference between a continuum and a narrow resonance mode having slightly different polarization response. In order to elucidate this, we first experimentally demonstrate an interferometric weak value amplification concept by generating nearly destructive interference of two paths of an interferometer having slightly rotated linear polarization states of light. The weak value amplification of polarization rotation effect is manifested as dramatic changes in the polarization state of light, which acts as the pointer. We go on to demonstrate that the manifestation of natural interferometric weak value amplification is an important contributing factor to the observed giant Faraday rotation and ellipticity in waveguided magneto-plasmonic crystals exhibiting prominent Fano resonance. The natural weak value interpretation of the enhanced Faraday rotation in hybrid magneto-plasmonic systems enriches the existing understanding on its origin. This opens up a new paradigm of natural weak measurement for gaining fundamental insights and ensuing practical applications on various weak interaction effects in rich variety of wave phenomena that originate from fine interference effects.

| S-EPMC7351789 | biostudies-literature

Crack-resistant Al2O3-SiO2 glasses.

Project description:Obtaining "hard" and "crack-resistant" glasses have always been of great important in glass science and glass technology. However, in most commercial glasses both properties are not compatible. In this work, colorless and transparent xAl2O3-(100-x)SiO2 glasses (30 ≤ x ≤ 60) were fabricated by the aerodynamic levitation technique. The elastic moduli and Vickers hardness monotonically increased with an increase in the atomic packing density as the Al2O3 content increased. Although a higher atomic packing density generally enhances crack formation in conventional oxide glasses, the indentation cracking resistance increased by approximately seven times with an increase in atomic packing density in binary Al2O3-SiO2 glasses. In particular, the composition of 60Al2O3 • 40SiO2 glass, which is identical to that of mullite, has extraordinary high cracking resistance with high elastic moduli and Vickers hardness. The results indicate that there exist aluminosilicate compositions that can produce hard and damage-tolerant glasses.

| S-EPMC4823710 | biostudies-other

A Closer Look on Nuclear Radiation Shielding Properties of Eu3+ Doped Heavy Metal Oxide Glasses: Impact of Al2O3/PbO Substitution.

Project description:In this study, a group of heavy metal oxide glasses with a nominal composition of 55B2O3 + 19.5TeO2 + 10K2O + (15-x) PbO + xAl2O3 + 0.5Eu2O3 (where x = 0, 2.5, 5, 7.5, 10, 12.5, and 15 in wt.%) were investigated in terms of their nuclear radiation shielding properties. These glasses containing lanthanide-doped heavy metal oxide were envisioned to yield valuable results in respect to radiation shielding, and thus a detailed investigation was carried out; the obtained results were compared with traditional and new generation shields. Advanced simulation and theoretical methods have been utilized in a wide range of energy regions. Our results showed that the AL0.0 sample with the highest PbO contribution had superior shielding properties in the entire energy range. The effective removal of cross-sections for fast neutrons (ΣR) was also examined. The results indicated that AL5.0 had the greatest value. While increasing the concentration of Al2O3 in samples had a negative effect on the radiation shielding characteristics, it can be concluded that using PbO in the Eu3+ doped heavy metal oxide glasses could be a useful tool to keep gamma-ray shielding properties at a maximum level.

| S-EPMC8466938 | biostudies-literature

Insights into Magneto-Optics of Helical Conjugated Polymers.

Project description:Materials with magneto-optic (MO) properties have enabled critical fiber-optic applications and highly sensitive magnetic field sensors. While traditional MO materials are inorganic in nature, new generations of MO materials based on organic semiconducting polymers could allow increased versatility for device architectures, manufacturing options, and flexible mechanics. However, the origin of MO activity in semiconducting polymers is far from understood. In this paper, we report high MO activity observed in a chiral helical poly-3-(alkylsulfone)thiophene (P3AST), which confirms a new design for the creation of a giant Faraday effect with Verdet constants up to (7.63 ± 0.78) × 104 deg T-1 m-1 at 532 nm. We have determined that the sign of the Verdet constant and its magnitude are related to the helicity of the polymer at the measured wavelength. The Faraday rotation and the helical conformation of P3AST are modulated by thermal annealing, which is further supported by DFT calculations and MD simulations. Our results demonstrate that helical polymers exhibit enhanced Verdet constants and expand the previous design space for polythiophene MO materials that was thought to be limited to highly regular lamellar structures. The structure-property studies herein provide insights for the design of next-generation MO materials based upon semiconducting organic polymers.

| S-EPMC5992603 | biostudies-literature

Na-Faraday rotation filtering: the optimal point.

Project description:Narrow-band optical filtering is required in many spectroscopy applications to suppress unwanted background light. One example is quantum communication where the fidelity is often limited by the performance of the optical filters. This limitation can be circumvented by utilizing the GHz-wide features of a Doppler broadened atomic gas. The anomalous dispersion of atomic vapours enables spectral filtering. These, so-called, Faraday anomalous dispersion optical filters (FADOFs) can be by far better than any commercial filter in terms of bandwidth, transition edge and peak transmission. We present a theoretical and experimental study on the transmission properties of a sodium vapour based FADOF with the aim to find the best combination of optical rotation and intrinsic loss. The relevant parameters, such as magnetic field, temperature, the related optical depth, and polarization state are discussed. The non-trivial interplay of these quantities defines the net performance of the filter. We determine analytically the optimal working conditions, such as transmission and the signal to background ratio and validate the results experimentally. We find a single global optimum for one specific optical path length of the filter. This can now be applied to spectroscopy, guide star applications, or sensing.

| S-EPMC4190536 | biostudies-other

Nonreciprocal surface acoustic wave propagation via magneto-rotation coupling.

Project description:A fundamental form of magnon-phonon interaction is an intrinsic property of magnetic materials, the "magnetoelastic coupling." This form of interaction has been the basis for describing magnetostrictive materials and their applications, where strain induces changes of internal magnetic fields. Different from the magnetoelastic coupling, more than 40 years ago, it was proposed that surface acoustic waves may induce surface magnons via rotational motion of the lattice in anisotropic magnets. However, a signature of this magnon-phonon coupling mechanism, termed magneto-rotation coupling, has been elusive. Here, we report the first observation and theoretical framework of the magneto-rotation coupling in a perpendicularly anisotropic film Ta/CoFeB(1.6 nanometers)/MgO, which consequently induces nonreciprocal acoustic wave attenuation with an unprecedented ratio of up to 100% rectification at a theoretically predicted optimized condition. Our work not only experimentally demonstrates a fundamentally new path for investigating magnon-phonon coupling but also justifies the feasibility of the magneto-rotation coupling application.

| S-EPMC7413730 | biostudies-literature

Faraday rotation echo spectroscopy and detection of quantum fluctuations.

Project description:Central spin decoherence is useful for detecting many-body physics in environments and moreover, the spin echo control can remove the effects of static thermal fluctuations so that the quantum fluctuations are revealed. The central spin decoherence approach, however, is feasible only in some special configurations and often requires uniform coupling between the central spin and individual spins in the baths, which are very challenging in experiments. Here, by making analogue between central spin decoherence and depolarization of photons, we propose a scheme of Faraday rotation echo spectroscopy (FRES) for studying quantum fluctuations in interacting spin systems. The echo control of the photon polarization is realized by flipping the polarization with a birefringence crystal. The FRES, similar to spin echo in magnetic resonance spectroscopy, can suppress the effects of the static magnetic fluctuations and therefore reveal dynamical magnetic fluctuations. We apply the scheme to a rare-earth compound LiHoF4 and calculate the echo signal, which is related to the quantum fluctuations of the system. We observe enhanced signals at the phase boundary. The FRES should be useful for studying quantum fluctuations in a broad range of spin systems, including cold atoms, quantum dots, solid-state impurities, and transparent magnetic materials.

| S-EPMC3986868 | biostudies-other

Strong interband Faraday rotation in 3D topological insulator Bi2Se3.

Project description:The Faraday effect is a representative magneto-optical phenomenon, resulting from the transfer of angular momentum between interacting light and matter in which time-reversal symmetry has been broken by an externally applied magnetic field. Here we report on the Faraday rotation induced in the prominent 3D topological insulator Bi2Se3 due to bulk interband excitations. The origin of this non-resonant effect, extraordinarily strong among other non-magnetic materials, is traced back to the specific Dirac-type Hamiltonian for Bi2Se3, which implies that electrons and holes in this material closely resemble relativistic particles with a non-zero rest mass.

| S-EPMC4707504 | biostudies-other

Perfect X-ray focusing via fitting corrective glasses to aberrated optics.

Project description:Due to their short wavelength, X-rays can in principle be focused down to a few nanometres and below. At the same time, it is this short wavelength that puts stringent requirements on X-ray optics and their metrology. Both are limited by today's technology. In this work, we present accurate at wavelength measurements of residual aberrations of a refractive X-ray lens using ptychography to manufacture a corrective phase plate. Together with the fitted phase plate the optics shows diffraction-limited performance, generating a nearly Gaussian beam profile with a Strehl ratio above 0.8. This scheme can be applied to any other focusing optics, thus solving the X-ray optical problem at synchrotron radiation sources and X-ray free-electron lasers.

| S-EPMC5337966 | biostudies-literature

OmicsDI is part of the ELIXIR infrastructure

OmicsDI is an Elixir interoperability service. Learn more ›

Tweets

OmicsDI Databases

PRIDE
PeptideAtlas
MassIVE
JPOST Repository
Physiome Model Repository

EGA
EVA
ENA
LINCS
PAXDB
Cell Collective

MetaboLights
Metabolomics Workbench
MetabolomeExpress
GNPS
BioModels
FAIRDOMHub

ArrayExpress
dbGaP
ExpressionAtlas
GEO
NODE

Information

Databases
Help
API
Contact us
Code on GitHub
Terms of use
Submit Data