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Overbias Photon Emission from Light-Emitting Devices Based on Monolayer Transition Metal Dichalcogenides.


ABSTRACT: Tunneling light-emitting devices (LEDs) based on transition metal dichalcogenides (TMDs) and other two-dimensional (2D) materials are a new platform for on-chip optoelectronic integration. Some of the physical processes underlying this LED architecture are not fully understood, especially the emission at photon energies higher than the applied electrostatic potential, so-called overbias emission. Here we report overbias emission for potentials that are near half of the optical bandgap energy in TMD-based tunneling LEDs. We show that this emission is not thermal in nature but consistent with exciton generation via a two-electron coherent tunneling process.

SUBMITTER: Shan S 

PROVIDER: S-EPMC10722526 | biostudies-literature | 2023 Dec

REPOSITORIES: biostudies-literature

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Overbias Photon Emission from Light-Emitting Devices Based on Monolayer Transition Metal Dichalcogenides.

Shan Shengyu S   Huang Jing J   Papadopoulos Sotirios S   Khelifa Ronja R   Taniguchi Takashi T   Watanabe Kenji K   Wang Lujun L   Novotny Lukas L  

Nano letters 20231204 23


Tunneling light-emitting devices (LEDs) based on transition metal dichalcogenides (TMDs) and other two-dimensional (2D) materials are a new platform for on-chip optoelectronic integration. Some of the physical processes underlying this LED architecture are not fully understood, especially the emission at photon energies higher than the applied electrostatic potential, so-called overbias emission. Here we report overbias emission for potentials that are near half of the optical bandgap energy in  ...[more]

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