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Green polymeric nanomaterials for the photocatalytic degradation of dyes: a review.

ABSTRACT: Pure and drinkable water will be rarer and more expensive as the result of pollution induced by industrialisation, urbanisation and population growth. Among the numerous sources of water pollution, the textile industry has become a major issue because effluents containing dyes are often released in natural water bodies. For instance, about two years are needed to biodegrade dye-derived, carcinogenic aromatic amines, in sediments. Classical remediation methods based upon physicochemical reactions are costly and still generate sludges that contain amine residues. Nonetheless, recent research shows that nanomaterials containing biopolymers are promising to degrade organic pollutants by photocatalysis. Here, we review the synthesis and applications of biopolymeric nanomaterials for photocatalytic degradation of azo dyes. We focus on conducting biopolymers incorporating metal, metal oxide, metal/metal oxide and metal sulphide for improved biodegradation. Biopolymers can be obtained from microorganisms, plants and animals. Unlike fossil-fuel-derived polymers, biopolymers are carbon neutral and thus sustainable in the context of global warming. Biopolymers are often biodegradable and biocompatible.

SUBMITTER: Sarkar S

PROVIDER: S-EPMC7293757 | biostudies-literature | 2020 Jun

REPOSITORIES: biostudies-literature

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Green polymeric nanomaterials for the photocatalytic degradation of dyes: a review.

Sarkar Shrabana S Ponce Nidia Torres NT Banerjee Aparna A Bandopadhyay Rajib R Rajendran Saravanan S Lichtfouse Eric E

Environmental chemistry letters 20200614 5

Pure and drinkable water will be rarer and more expensive as the result of pollution induced by industrialisation, urbanisation and population growth. Among the numerous sources of water pollution, the textile industry has become a major issue because effluents containing dyes are often released in natural water bodies. For instance, about two years are needed to biodegrade dye-derived, carcinogenic aromatic amines, in sediments. Classical remediation methods based upon physicochemical reactions ...[more]

PMID: 32837482

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Project description:Immobilization of inorganic metal quantum dots (especially, noble transition metals) onto organic polymers to synthesize nanometal-polymer composites (NMPCs) has attracted considerable attention because of their advanced optical, electrical, catalytic/photocatalytic, and biological properties. Herein, novel, highly efficient, stable, and visible light-active NMPC photocatalysts consisting of silver quantum dots (Ag QDs) immobilized onto polymeric chitosan-polyethylene oxide (CTS-PEO) blend sheets have been successfully prepared by an in situ self-assembly facile casting method as a facile and green approach. The CTS-PEO blend polymer acts as a reducing and a stabilizing agent for Ag QDs which does not generate any environmental chemical pollutant. The prepared x wt % Ag QDs/CTS-PEO composites were fully characterized through X-ray diffraction, Fourier transform infrared spectroscopy, transmission electron microscopy (TEM), thermogravimetric analysis, and UV/visible spectroscopy. The characterization results indicated the successful synthesis of the Ag QDs/CTS-PEO composites by the interactions and complexation between x wt % Ag QDs and CTS-PEO blend sheets. TEM images revealed small granules randomly distributed onto the CTS-PEO blend sheets, indicating the immobilization of Ag QDs onto CTS-PEO composites. The presence of a surface plasmon resonance (SPR) band and the shifting of the absorption edge toward higher wavelengths in the UV/vis spectra indicated the formation of x wt % Ag QDs/CTS-PEO composites. The Ag QDs in the polymeric blend matrix led to remarkable enhancement in the optical, thermal, electrical, and photocatalytic properties of x wt % Ag QDs/CTS-PEO composites. The photocatalytic efficiency of the prepared composites was evaluated by the photodegradation of p-nitrophenol (PNP) under simulated sunlight. The maximum photocatalytic degradation reached 91.1% efficiency within 3 h for the 12.0 wt % Ag QDs/CTS-PEO photocatalyst. Generally, the Ag QDs immobilized onto CTS-PEO blend composites significantly enhance the SPR effect and the synergistic effect and reduce the band gap, leading to a high photocatalytic activity.

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Green polymeric nanomaterials for the photocatalytic degradation of dyes: a review.

Publications

Green polymeric nanomaterials for the photocatalytic degradation of dyes: a review.

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