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Stratospheric intrusion-influenced ozone air quality exceedances investigated in the NASA MERRA-2 Reanalysis.

ABSTRACT: Stratospheric intrusions have been the interest of decades of research for their ability to bring stratospheric ozone (O3) into the troposphere with the potential to enhance surface O3 concentrations. However, these intrusions have been misrepresented in models and reanalyses until recently, as the features of a stratospheric intrusion are best identified in horizontal resolutions of 50 km or smaller. NASA's Modern-Era Retrospective Analysis for Research and Applications Version-2 (MERRA-2) reanalysis is a publicly-available high-resolution dataset (~50 km) with assimilated O3 that characterizes O3 on the same spatiotemporal resolution as the meteorology. We demonstrate the science capabilities of the MERRA-2 reanalysis when applied to the evaluation of stratospheric intrusions that impact surface air quality. This is demonstrated through a case study analysis of stratospheric intrusion-influenced O3 exceedences in spring 2012 in Colorado, using a combination of observations, the MERRA-2 reanalysis and the Goddard Earth Observing System Model, Version 5 (GEOS-5) simulations.

SUBMITTER: Knowland KE

PROVIDER: S-EPMC7370994 | biostudies-literature | 2017 Sep

REPOSITORIES: biostudies-literature

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Stratospheric intrusion-influenced ozone air quality exceedances investigated in the NASA MERRA-2 Reanalysis.

Knowland K E KE Ott L E LE Duncan B N BN Wargan K K

Geophysical research letters 20170901 20

Stratospheric intrusions have been the interest of decades of research for their ability to bring stratospheric ozone (O<sub>3</sub>) into the troposphere with the potential to enhance surface O<sub>3</sub> concentrations. However, these intrusions have been misrepresented in models and reanalyses until recently, as the features of a stratospheric intrusion are best identified in horizontal resolutions of 50 km or smaller. NASA's Modern-Era Retrospective Analysis for Research and Applications Ve ...[more]

PMID: 32692318

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Project description:The representation of upper tropospheric/lower stratospheric (UTLS) jet and tropopause characteristics is compared in five modern high-resolution reanalyses for 1980 through 2014. Climatologies of upper tropospheric jet, subvortex jet (the lowermost part of the stratospheric vortex), and multiple tropopause frequency distributions in MERRA (Modern Era Retrospective Analysis for Research and Applications), ERA-I (the ECMWF interim reanalysis), JRA-55 (the Japanese 55-year Reanalysis), and CFSR (the Climate Forecast System Reanalysis) are compared with those in MERRA-2. Differences between alternate products from individual reanalysis systems are assessed; in particular, a comparison of CFSR data on model and pressure levels highlights the importance of vertical grid spacing. Most of the differences in distributions of UTLS jets and multiple tropopauses are consistent with the differences in assimilation model grids and resolution: For example, ERA-I (with coarsest native horizontal resolution) typically shows a significant low bias in upper tropospheric jets with respect to MERRA-2, and JRA-55 a more modest one, while CFSR (with finest native horizontal resolution) shows a high bias with respect to MERRA-2 in both upper tropospheric jets and multiple tropopauses. Vertical temperature structure and grid spacing are especially important for multiple tropopause characterization. Substantial differences between MERRA and MERRA-2 are seen in mid- to high-latitude southern hemisphere winter upper tropospheric jets and multiple tropopauses, and in the upper tropospheric jets associated with tropical circulations during the solstice seasons; some of the largest differences from the other reanalyses are seen in the same times and places. Very good qualitative agreement among the reanalyses is seen between the large scale climatological features in UTLS jet and multiple tropopause distributions. Quantitative differences may, however, have important consequences for transport and variability studies. Our results highlight the importance of considering reanalyses differences in UTLS studies, especially in relation to resolution and model grids; this is particularly critical when using high-resolution reanalyses as an observational reference for evaluating global chemistry climate models.

Dataset Information

Stratospheric intrusion-influenced ozone air quality exceedances investigated in the NASA MERRA-2 Reanalysis.

Publications

Stratospheric intrusion-influenced ozone air quality exceedances investigated in the NASA MERRA-2 Reanalysis.

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