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Investigation of the Effect of Nanoparticle-Stabilized Foam on EOR: Nitrogen Foam and Methane Foam.

ABSTRACT: In recent years, studies conducted on foam stabilization have focused on nanoparticles by generating strong adsorption at the interface to stabilize the foam under harsh reservoir conditions. Meanwhile, the selection of a gas source is also of great importance for foam performance. In this study, a mixed system of surfactants was selected, and the foamability and foam stability of nitrogen and methane were evaluated according to the improved jet method. After adding modified SiO2 nanoparticles, the foam-related parameters were analyzed. The plugging abilities of the different foams were compared through core-flooding experiments, and the oil displacement effects of the different foams were compared through microfluidic experiments. The results show that the amphoteric surfactant betaine has an excellent synergistic effect on the anionic surfactant SDS. The methane foam produced using the jet method has a larger initial volume than the nitrogen foam, but its stability is poor. The half-life of the nitrogen foam is about two times that of the methane foam. After adding 1.0 wt % SiO2 nanoparticles to the surfactant solution, the viscosity and stability of the formed foam improve. However, the maximum viscosity of the surfactant nanoparticle foam (surfactant-NP foam) is 53 mPa·s higher than that of the surfactant foam. In the core-flooding experiment, the plugging performance of the methane foam was worse than that of the nitrogen foam, and in the microfluidic experiment, the oil displacement abilities of the methane foam and the nitrogen foam were similar. The plugging performance and the oil displacement effect of the foam are greatly improved by adding nanoparticles. The surfactant-NP foam flooding has a better oil displacement effect and can enhance the recovery factor by more than 30%. Under actual high-pressure reservoir conditions, although the stability of the methane foam is weaker than that of the nitrogen foam, some methane may be dissolved in the crude oil to decrease the viscosity after the foam collapses, which leads to the methane foam being the preferred method in oilfields.

SUBMITTER: Xu Z

PROVIDER: S-EPMC7408255 | biostudies-literature | 2020 Aug

REPOSITORIES: biostudies-literature

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Investigation of the Effect of Nanoparticle-Stabilized Foam on EOR: Nitrogen Foam and Methane Foam.

Xu Zhengxiao Z Li Binfei B Zhao Haiyang H He Long L Liu Zhiliang Z Chen Danqi D Yang Huiyu H Li Zhaomin Z

ACS omega 20200723 30

In recent years, studies conducted on foam stabilization have focused on nanoparticles by generating strong adsorption at the interface to stabilize the foam under harsh reservoir conditions. Meanwhile, the selection of a gas source is also of great importance for foam performance. In this study, a mixed system of surfactants was selected, and the foamability and foam stability of nitrogen and methane were evaluated according to the improved jet method. After adding modified SiO<sub>2</sub> nano ...[more]

PMID: 32775911

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Project description:Cellulose nanocrystals (CNCs) and 2,2,6,6-tetramethylpiperidine-1-oxyl (TEMPO)-oxidized cellulose nanofibrils (T-CNFs) were tested as enhanced oil recovery (EOR) agents through core floods and microfluidic experiments. Both particles were mixed with low salinity water (LSW). The core floods were grouped into three parts based on the research objectives. In Part 1, secondary core flood using CNCs was compared to regular water flooding at fixed conditions, by reusing the same core plug to maintain the same pore structure. CNCs produced 5.8% of original oil in place (OOIP) more oil than LSW. For Part 2, the effect of injection scheme, temperature, and rock wettability was investigated using CNCs. The same trend was observed for the secondary floods, with CNCs performing better than their parallel experiment using LSW. Furthermore, the particles seemed to perform better under mixed-wet conditions. Additional oil (2.9-15.7% of OOIP) was produced when CNCs were injected as a tertiary EOR agent, with more incremental oil produced at high temperature. In the final part, the effect of particle type was studied. T-CNFs produced significantly more oil compared to CNCs. However, the injection of T-CNF particles resulted in a steep increase in pressure, which never stabilized. Furthermore, a filter cake was observed at the core face after the experiment was completed. Microfluidic experiments showed that both T-CNF and CNC nanofluids led to a better sweep efficiency compared to low salinity water flooding. T-CNF particles showed the ability to enhance the oil recovery by breaking up events and reducing the trapping efficiency of the porous medium. A higher flow rate resulted in lower oil recovery factors and higher remaining oil connectivity. Contact angle and interfacial tension measurements were conducted to understand the oil recovery mechanisms. CNCs altered the interfacial tension the most, while T-CNFs had the largest effect on the contact angle. However, the changes were not significant enough for them to be considered primary EOR mechanisms.

Dataset Information

Investigation of the Effect of Nanoparticle-Stabilized Foam on EOR: Nitrogen Foam and Methane Foam.

Publications

Investigation of the Effect of Nanoparticle-Stabilized Foam on EOR: Nitrogen Foam and Methane Foam.

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