Steam condensation heat transfer on lubricant-infused surfaces.
Ontology highlight
ABSTRACT:
SUBMITTER: Stoddard R
PROVIDER: S-EPMC8050781 | biostudies-literature |
REPOSITORIES: biostudies-literature
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Project description:Water vapor condensation is common in nature and widely used in industrial applications, including water harvesting, power generation, and desalination. As compared to traditional filmwise condensation, dropwise condensation on lubricant-infused surfaces (LIS) can lead to an order-of-magnitude increase in heat transfer rates. Small droplets (D ? 100 ?m) account for nearly 85% of the total heat transfer and droplet sweeping plays a crucial role in clearing nucleation sites, allowing for frequent re-nucleation. Here, we focus on the dynamic interplay of microdroplets with the thin lubricant film during water vapor condensation on LIS. Coupling high-speed imaging, optical microscopy, and interferometry, we show that the initially uniform lubricant film re-distributes during condensation. Governed by lubricant height gradients, microdroplets as small as 2 ?m in diameter undergo rigorous and gravity-independent self-propulsion, travelling distances multiples of their diameters at velocities up to 1100 ?m s-1. Although macroscopically the movement appears to be random, we show that on a microscopic level capillary attraction due to asymmetrical lubricant menisci causes this gravity-independent droplet motion. Based on a lateral force balance analysis, we quantitatively find that the sliding velocity initially increases during movement, but decreases sharply at shorter inter-droplet spacing. The maximum sliding velocity is inversely proportional to the oil viscosity and is strongly dependent of the droplet size, which is in excellent agreement with the experimental observations. This novel and non-traditional droplet movement is expected to significantly enhance the sweeping efficiency during dropwise condensation, leading to higher nucleation and heat transfer rates.
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Project description:Recently, lubricant-impregnated surfaces (LIS) have emerged as a promising condenser surface by facilitating the removal of condensates from the surface. However, LIS has the critical limitation in that lubricant oil is depleted along with the removal of condensates. Such oil depletion is significantly aggravated under high condensation heat transfer. Here we propose a brushed LIS (BLIS) that can allow the application of LIS under high condensation heat transfer indefinitely by overcoming the previous oil depletion limit. In BLIS, a brush replenishes the depleted oil via physical contact with the rotational tube, while oil is continuously supplied to the brush by capillarity. In addition, BLIS helps enhance heat transfer performance with additional route to droplet removal by brush sweeping. By applying BLIS, we maintain the stable dropwise condensation mode for?>?48?hours under high supersaturation levels along with up to 61% heat transfer enhancement compared to hydrophobic surfaces.
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Project description:Enhancing condensation heat transfer is important for broad applications from power generation to water harvesting systems. Significant efforts have focused on easy removal of the condensate, yet the other desired properties of low contact angles and high nucleation densities for high heat transfer performance have been typically neglected. In this work, we demonstrate immersion condensation on oil-infused micro and nanostructured surfaces with heterogeneous coatings, where water droplets nucleate immersed within the oil. The combination of surface energy heterogeneity, reduced oil-water interfacial energy, and surface structuring enabled drastically increased nucleation densities while maintaining easy condensate removal and low contact angles. Accordingly, on oil-infused heterogeneous nanostructured copper oxide surfaces, we demonstrated approximately 100% increase in heat transfer coefficient compared to state-of-the-art dropwise condensation surfaces in the presence of non-condensable gases. This work offers a distinct approach utilizing surface chemistry and structuring together with liquid-infusion for enhanced condensation heat transfer.
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Project description:Slippery lubricant-infused surfaces (SLIPS) have shown great promise for anti-frosting and anti-icing. However, small length scales associated with frost dendrites exert immense capillary suction pressure on the lubricant. This pressure depletes the lubricant film and is detrimental to the functionality of SLIPS. To prevent lubricant depletion, we demonstrate that interstitial spacing in SLIPS needs to be kept below those found in frost dendrites. Densely packed nanoparticles create the optimally sized nanointerstitial features in SLIPS (Nano-SLIPS). The capillary pressure stabilizing the lubricant in Nano-SLIPS balances or exceeds the capillary suction pressure by frost dendrites. We term this concept capillary balancing. Three-dimensional spatial analysis via confocal microscopy reveals that lubricants in optimally structured Nano-SLIPS are not affected throughout condensation (0 °C), extreme frosting (-20 °C to -100 °C), and traverse ice-shearing (-10 °C) tests. These surfaces preserve low ice adhesion (10-30 kPa) over 50 icing cycles, demonstrating a design principle for next-generation anti-icing surfaces.
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Project description:Icephobic coating and surfaces are essential for protecting infrastructures such as transmission lines, transportation vehicles, and many others from severe damages of excessive icing. The slippery liquid-infused porous surfaces (SLIPS) are attracting escalating attention because of their low-ice adhesion strength. Despite all of the encouraging laboratory scale results, the SLIPS are still far from being applicable in real environments owing to the key unsolved problem, namely anti-icing durability. Inspired by the functionality of the amphibians' skin, lubricant regenerability was introduced to conventional SLIPS and realized by a facile and scalable fabrication route. A series of polydimethylsiloxane (PDMS)-based skinlike SLIPS were designed and fabricated by using a one-step method, the solvent evaporation-induced phase separation technique. The obtained skinlike SLIPS were able to regenerate surface lubricant constantly by internal residual stress because of phase separation and survive more than 15 cycles of wiping/regenerating tests. Thanks to the regenerability of the surface lubricant, the new SLIPS demonstrated durable icephobicity, showing a long-term low-ice adhesion strength below 70 kPa, which was only 43% of 160 kPa that for the pristine PDMS (Sylgard 184), even after 15 icing/deicing cycles. This work paves a new and facile way for achieving icephobic durability of SLIPS.
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Project description:Heterogeneous surfaces with wetting contrast have gained extensive attention in recent years because of their potential application in condensation heat transfer enhancement. In this work, we engineered superhydrophobic/hydrophilic hybrid (SHH) surfaces on copper substrates via a laser-ablation process. We demonstrated that the as-fabricated SHH surfaces present dropwise condensation behavior; the condensate droplet growth, departure, and heat transfer performance depend strongly on the spacing of the hydrophilic spot. The surface with the hydrophilic spot spacing of 100 μm (SHH100) exhibits the most efficient dropwise condensation in terms of fast droplet growth rate, efficient coalescence-induced droplet departure, as well as enhanced heat transfer coefficient (HTC) compared to the homogeneous superhydrophobic (SHPo) surface. The mechanism underlying the enhanced condensation heat transfer performance is analyzed. A 12% enhancement on condensation HTC was found was found on SHH100 surface compared with the SHPo surface. Our results provide important insights for the design of hybrid surfaces with wetting contrast for enhancing condensation heat transfer performance in many industrial applications.
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Project description:Condensation of water from the atmosphere on a solid surface is an ubiquitous phenomenon in nature and has diverse technological applications, e.g. in heat and mass transfer. We investigated the condensation kinetics of water drops on a lubricant-impregnated surface, i.e., a micropillar array impregnated with a non-volatile ionic liquid. Growing and coalescing drops were imaged in 3D using a laser scanning confocal microscope equipped with a temperature and humidity control. Different stages of condensation can be discriminated. On a lubricant-impregnated hydrophobic micropillar array these are: (1) Nucleation on the lubricant surface. (2) Regular alignment of water drops between micropillars and formation of a three-phase contact line on a bottom of the substrate. (3) Deformation and bridging by coalescence which eventually leads to a detachment of the drops from the bottom substrate. The drop-substrate contact does not result in breakdown of the slippery behaviour. Contrary, on a lubricant-impregnated hydrophilic micropillar array, the condensed water drops replace the lubricant. Consequently, the surface loses its slippery property. Our results demonstrate that a Wenzel-like to Cassie transition, required to maintain the facile removal of condensed water drops, can be induced by well-chosen surface hydrophobicity.
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Project description:Enhancement in heat-transfer performance via dropwise condensation on superhydrophobic surfaces is much greater than that realized via generic condensation on a regular surface. However, if the supersaturation level during condensation increases above a specific value, water may seep to greater depths between structures. This may lead to attached condensation, which reduces condensation heat-transfer efficiency below that of ordinary surfaces. Therefore, it is critical to avoid the occurrence of supersaturation when superhydrophobic surfaces are employed in condenser design. The proposed study presents a simple method for regulating supersaturation on the laboratory scale. Experiments concerning droplet behavior on a superhydrophobic plate were performed to investigate droplet detachment and attachment in accordance with the surface and droplet temperatures. Results obtained have been represented as a ″droplet-behavior map″, which clearly depicts boundaries dividing the detachment and attachment regions. The supersaturation threshold obtained from the said map has been compared against results obtained from condensation heat-transfer experiments performed in an actual condenser environment. As observed, the two results demonstrate excellent agreement. Although superhydrophobicity of surfaces remains unchanged at room temperature, changes may occur in the extent of the supersaturation section, which improves condensation heat-transfer performance, depending on the surface-structure complexity. Therefore, droplet-behavior mapping has been used in this study to determine the available supersaturation section in accordance with the variation in surface roughness. Results confirm that the available supersaturation region increases with increasing surface roughness and structural complexity. Therefore, prior to applying superhydrophobicity to condensers, droplet-behavior mapping must be performed to avoid operation under the supersaturation conditions, which causes attached condensation.
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