Ontology highlight
ABSTRACT:
SUBMITTER: Dorfman KE
PROVIDER: S-EPMC4141681 | biostudies-literature | 2014 Aug
REPOSITORIES: biostudies-literature
Dorfman Konstantin E KE Schlawin Frank F Mukamel Shaul S
The journal of physical chemistry letters 20140711 16
We propose a novel femtosecond stimulated Raman spectroscopy (FSRS) technique that combines entangled photons with interference detection to select matter pathways and enhance the resolution. Following photoexcitation by an actinic pump, the measurement uses a pair of broad-band entangled photons; one (signal) interacts with the molecule and together with a third narrow-band pulse induces the Raman process. The other (idler) photon provides a reference for the coincidence measurement. This inter ...[more]