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Atomic Scale Modulation of Self-Rectifying Resistive Switching by Interfacial Defects.


ABSTRACT: Higher memory density and faster computational performance of resistive switching cells require reliable array-accessible architecture. However, selecting a designated cell within a crossbar array without interference from sneak path currents through neighboring cells is a general problem. Here, a highly doped n++ Si as the bottom electrode with Ni-electrode/HfO x /SiO2 asymmetric self-rectifying resistive switching device is fabricated. The interfacial defects in the HfO x /SiO2 junction and n++ Si substrate result in the reproducible rectifying behavior. In situ transmission electron microscopy is used to quantitatively study the properties of the morphology, chemistry, and dynamic nucleation-dissolution evolution of the chains of defects at the atomic scale. The spatial and temporal correlation between the concentration of oxygen vacancies and Ni-rich conductive filament modifies the resistive switching effect. This study has important implications at the array-level performance of high density resistive switching memories.

SUBMITTER: Wu X 

PROVIDER: S-EPMC6010905 | biostudies-other | 2018 Jun

REPOSITORIES: biostudies-other

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Atomic Scale Modulation of Self-Rectifying Resistive Switching by Interfacial Defects.

Wu Xing X   Yu Kaihao K   Cha Dongkyu D   Bosman Michel M   Raghavan Nagarajan N   Zhang Xixiang X   Li Kun K   Liu Qi Q   Sun Litao L   Pey Kinleong K  

Advanced science (Weinheim, Baden-Wurttemberg, Germany) 20180414 6


Higher memory density and faster computational performance of resistive switching cells require reliable array-accessible architecture. However, selecting a designated cell within a crossbar array without interference from sneak path currents through neighboring cells is a general problem. Here, a highly doped n<sup>++</sup> Si as the bottom electrode with Ni-electrode/HfO <i><sub>x</sub></i> /SiO<sub>2</sub> asymmetric self-rectifying resistive switching device is fabricated. The interfacial de  ...[more]

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